Stochastic coupling and thermodynamic inequalities

Let ₁ and ₂ be thermodynamic Gibbs measures on ^m and ⁿ , respectively. Diffusions are constructed having ₁, and ₂ as invariant measures. These diffusions are then coupled; inequalities between expectations of certain random variables on the two spaces result.Partially supported by NSF-MCS 74-07313-A03     

New cw fir laser emissions from CO2 laser-pumped vinyl bromide

47 new cw far-infrared laser lines with wavelenths between 453 and 2356 m have been obtained by optically pumping vinyl bromide (C₂H₃Br) by a CO₂ laser. A significant portion of these lines has wavelengths longer than 750 m.     

Time delays in lead-salt semiconductor diode lasers

Time delays of typically 15–17 have been measured directly for PbS_1–xSe_x, Pb_1–xSn_xSe and Pb_1–xSn_xTe diode lasers at injection levels just above threshold in each case. The corresponding minority carrier lifetimes, as determined using the one-carrier injection model, were typically 2–4.     

Optically pumped14NH3 laser and its stark tuning at 10.78 μm

Infrared (ir) emissions from a TEA-CO₂-laser-pumped NH₃ laser are reported. Superfluorescent emissions and selective single-line oscillations have been obtained in the range from 11 to 13 m. The results make possible the design of a NH₃ Stark cell allowing a 1 GHz shift of the 10.78 m NH₃ emission line.     

Effect of Multi-Mode Optically Pumped Far-Infrared Laser Cavity on Spectra and Multi-Raman Interaction

Based on semi-classical density matrix theory, the spectral characteristics and multi-Raman interaction of multi-longitudinal-mode CO₂-9R(30) optically pumped cavity NH₃ molecules 67.2 m far-infrared laser were theoretically studied. And with different parameters such as input and output reflection coefficient, length of tube and so on, the rules of multi-Raman interaction and effect on longitudinal structure of 67.2 m far-infrared laser spectrum were also discussed theoretically.     

Systematic study of muon transfer to sulphur dioxide

In a systematic study of the transfer process to sulphur dioxide, in seven different H₂ + SO₂ gas mixtures, the time spectra of the muonic sulphur X-rays yield muon transfer rates to the SO₂ molecule, deduced from the lifetimes of the p atoms, which agree all well with each other. The muonic oxygen time spectra show an additional structure as if p atoms of another kind were present. Reduced transfer rates_O are reproducible if one uses the model of ephemeral p atoms. The intensity ratios between the different kinds of p atoms are also discussed in the framework of this model and the one of black and white p atoms.     

Finite-element thermal model for buried-heterostructure diode lasers

First results of our new finite-element modelling of thermal properties of GaAs/(AlGa)As buried-heterostructure (BH) lasers are reported. The calculus procedure is very efficient, so we have used a standard IBM PC/XT microcomputer. For the stripe active-region width of 1 m, the thermal resistance of the laser was determined to be about 70 KW^-1, whereas its electrical resistance was about 6 ohms. To the best of our knowledge, isothermal lines within BH lasers have been obtained for the first time. The isothermal configuration enables us to analyse heat-spreading phenomena in BH lasers, which makes possible thermal optimization of the laser construction.As the first application of the model, the relative influence of the oxide layer thickness on the laser thermal resistance was examined. Because of relatively large lateral dimensions of the laser crystal as compared to the active region, this influence is often neglected, whereas our detailed calculations reveal its importance. An increase in this thickness from 0.1 m to 0.5 m is followed by over 15% increase in the laser thermal resistance.     

Radiation Source in the Ranges 2.1–2.3 and 3.7–4.3 μm for the Spectroscopy of the Atmosphere

To expand the possibilities of spectroscopic systems based on a CO₂ laser, we have mixed the frequencies of its radiation with the radiation of erbium lasers. Simultaneous use of Er³⁺:CaF₂ ( = 2.76 m) and Er³⁺:YAG lasers ( = 2.96 m) makes it possible for the spectrum of generated sum and difference frequencies to overlap the ranges 2.2–2.3 and 3.6–4.3 m that coincide with the atmospheric transparency windows. Generation of the difference frequencies of radiation of erbium lasers and of the 10.6-m radiation of a CO₂ laser were observed in CdSe at a phase-matching angle of 72°40. In a bleached CdSe crystal of length 40 mm the efficiency of transformation has attained 12%. To sum up the frequencies, 4.5-mm ZnGeP₂ crystals were used, with the efficiency of transformation being 3% and the phase-matching angle being equal to 52°.     

Excited states of the molecular ion (H2μ)+

The rotation-vibration spectrum of (H₂ )⁺ is computed. Radiative lifetimes of the excited states are of order 10^–4 s or more. These times can be considered infinite compared to the lifetime of ⁺. For the ion in a crystal the lifetimes are significantly decreased by interaction with polarized molecules of the lattice. Transition rates to the ground state are calculated for (H₂ )⁺ in a hydrogen crystal. The results make it possible to interpret the experimental data from SR investigations of hydrogen, deuterium and hydrogen-deuterium mixtures.     

Q-switched Yb 3+ :YVO 4 laser with Raman self-conversion

We report the efficient continuous-wave (CW) and Q-switched laser operation of a diode-pumped Yb:YVO₄ laser. A CW output power of 1 W with a slope efficiency of 59% with respect to absorbed pump power was demonstrated. Passively Q-switched with a Cr⁴⁺:YAG saturable absorber, a Yb:YVO₄ laser with Raman conversion was demonstrated. Q-switched 18.7- J pulses with a pulse duration of 17 ns and a peak power up to 1 kW were obtained at 1018-nm fundamental wavelength and 3.6- J pulses with a pulse duration of 6 ns and a peak power of about 0.6 kW were obtained at 1119.5-nm first-Stokes wavelength.This revised version was published online in March 2005. In the previous version, the published online date was missing     

Isotope dependence of particle-decay rates of muonic molecular ions (d3,4Heμ) J=1 below (dμ)1s-3,4He threshold

Rates of particle-emitting decay of the resonant state of the muonic molecular ion (dHe) _J=1 lying below the (d)_1s-He threshold can decay to the d-He scattering state. The resonant state is estimated by scattering calculations with the non-adiabatic coupled-rearrangement-channel method. Strong isotope dependence of the decay rates of (d³He) _J=1 and (d⁴He) _J=1 is predicted, though the calculated radiative decay rates of the states are almost the same. In (d³He) _J=1, the particle decay width is three times larger than the radiative decay width, while the two types of decay widths are almost the same in (d⁴He) _J=1. This results in a strong hindrance of the branching ratio of the radiative decay of (d³He) _J=1 compared with the case of (d⁴He) _J=1. This is consistent with a recent observation of the radiative decay of the two molecular states.     

Slow and monoenergetic (3Heμ−)+ beam production and novel applications

Based upon the recent discovery at UT MSL/KEK, a new idea is proposed for producing a slow and monoenergetic (3.2 keV) (³He^–)⁺ ion beam by using particle decay of the (d³He) muon molecule formed during the (d) to³He transfer reaction. The proposed intense (³He) beam as well as the less intense (⁴He) beam will open up way to various new types of important CF experiments.     

Positron mobility in polyethylene in the 60–400 K temperature range

We have determined the positron mobility (₊) in polyethylene samples (67.2% crystalline, glass transition temperatureT _g=151 K) in the 64–400 K temperature range by Doppler shift measurements. A method based on the simulataneous observation of two lines from¹³³Ba and¹³⁷Cs radioactive sources together with the positron annihilation line, was employed to measure the Doppler shift of the 511 keV line as a function of the electric field applied to the samples. With this method we were able to measure at the same time the drift velocity of positrons and theS parameter. This parameter is very important in the interpretation of the mobility trend in samples where the positron states change with temperature. The positron mobility was corrected for positronium formation. ₊ at 64 K is 31.7±0.8 cm² V^–1 s^–1 then decreases up to 123 K, increases at 148 K and decreases again up to 170 K (₊=26.9±0.8 cm² V^–s^–). This sharp change in mobility is centred around the glass transition temperature of our samples. Then the mobility remains almost constant up to 230 K. From 250 K to 377 K, ₊ increases and reaches the value of 38.4±1.0 cm² V^–1s^–1. The corrected experimental data were well fitted by a simple model taking into account scattering and a thermally activated process (hopping mechanism).     

Magnetic moments of Gd nuclei

Low temperature nuclear orientation experiments down to 2 mK on¹⁴⁷GdFe,¹⁴⁹GdFe,¹⁴⁹GdGd and¹⁵³GdGd have yielded the magnetic hyperfine interaction strength. Bhf as 31.0(1.6) _NT, 28.3(2.0) _NT, 33.8(4.7) _NT and 13.3(2.1) _NT respectively. From these values the respective ground state magnetic moments ¦¦ of¹⁴⁷Gd,¹⁴⁹Gd and¹⁵⁹Gd were deduced as 1.12(20) _N, 1.01(16) _N and 0.40(8) _N.     

Experimental survey of the sticking problem in muon catalyzed dt fusion

The sticking process dt + n, which constitutes the most severe limit to the number of fusions which a muon can catalyze, is reviewed. Many attempts were made to determine by calculations and measurements the probability for initial sticking _s ⁰ (immediately after dt fusion) and for final sticking _s (after the came to rest). Previous results based on neutron disappearance rates and on the observation of -X-rays were controversial and also in some disagreement with theory. New data are reported from PSI on direct observation of final sticking, using a setup with the St. Petersburg ionization chamber. These data mark a significant improvement in reliability and may clarify questions concerning previous discrepancies. The new results is _s(0.56±0.04)%, lower than the theory prediction _s=(0.65±0.03)%, at medium density.     

Further investigations on ir pumping of CH3OD and CD3OD by a cw CO2 laser

Respectively, 41 and 36 new cw far-infrared lasing lines have been observed using a waveguide resonator in CH₃OD and CD₃OD pumped by a low-pressure CO₂ laser emitting in the 9.4, 10.4 m regular bands and in the 10.8 m hot band. The wavelength range was 46.6 m–1.67 mm in CH₃OD and 53.6 m–1 mm in CD₃OD.     

The influence of graphite boat material on the purity of LPE InGaAs

This paper describes the purity of LPE InGaAs layers grown in graphite boats, machined from various graphite materials. The influence of the material is clearly visible if the growth solution is sufficiently pure. Carrier concentrations n<2×l0¹⁵ cm^–3 and mobilities(77 K)> 38000 cm²/Vs are routinely achieved for suitable graphite materials already from the third run of a new large boat applying a prebake of only 15 h. Small boats yield even better results (n=0.5×10¹⁵ cm^–3 and(77 K)=49500 m²/Vs). The sticking of In-rich solutions to the graphite does not depend on the material but is solely dependent on the surface roughness. The problem of graphite particle abrasion is discussed.     

Harmonic coincidences between cw gas laser lines for extending frequency measurements to the 10μm wavelength region

Wavelength and frequency data for far-infrared c.w. gas laser lines have been scanned using a computer for chains of harmonic coincidences suitable for transferring frequency measurements from the submillimetre to the 10m wavelength region. A table of selected possibilities using up to three lasers in sequence is presented showing the calculated beat frequencies.     

μSR studies in the heavy fermion systems UNi2Al3, UPd2Al3 and U2PtC2

We have performed Muon Spin Relaxation (SR) measurements of several heavy fermion systems: UNi₂Al₃ (single crystal), UPd₂Al₃ (single crystal) and U₂PtC₂ (polycrystal). ZF -SR measurements of UNi₂Al₃ show magnetic order below the Néel temperatureT _N=4.6K, with the muon precession frequency(T 0)=2.5MHz at low temperatures. The local field distribution obtained at low temperatures in UNi₂Al₃ resembles that of the incommensurate spin density wave (SDW) system (TMTSF)₂PF₆, suggesting an incommensurate spin arrangement in UNi₂Al₃. TF -SR measurements give the penetration depth(T 0)=6100Å for UPd₂Al₃ and(T 0)=7000Å for U₂PtC₂ respectively. Since UPd₂Al₃ and U₂PtC₂ are clean superconductors (/l-0), we can combine n _s/m^* with the Sommerfeld constant n _s ^1/3 m^* to calculate the Fermi temperatureT _F ^3/4–1/4, which represents the characteristic energy scale of the superconducting carriers. We obtainT _C/T_F 0.01 for both UPd₂Al₃ and U₂PtC₂, comparable to other exotic superconductors, but quite different from simple metal BCS superconductors, whereT _C/T_F 0.01.     

Measurement of Optical Constants of CVD-Diamond for Short-Wavelength Far-Infrared Lasers

A diagnostic system using short-wavelength far-infrared (FIR) lasers (40–70 m in wavelength) is now being developed for high density and large volume plasmas. In the wavelength region, a CVD-diamond is the excellent materials for optical windows of the laser and the plasma vessel and beam splitters of a multichannel interferometer. To design these optical elements, the optical constants (refractive index n, absorption coefficient and transmissivity T) of the CVD-diamond have been measured precisely by using FIR lasers of 48-, 57- and 71-m in wavelength. As an example, the result for 57.1511 m light is n = 2.383(1) ± 0.002, = 0.19 ± 0.05 cm^-1 and T = 97.5 ± 1.5% at 1.023 mm in thickness.