Diamond‐based concept for combining beams at very high average powers

Ever since the laser's invention, there has been great interest in increasing beam output power without detriment to its coherence. Despite great advances having been obtained through the use of a diverse range of approaches, steady‐state beam powers above ten kilowatts remain a significant challenge for solid‐state lasers due to the heightened impact of detrimental nonlinear effects such as thermal lensing. Multiplexing several lasers using beam combination represents a method for surpassing the power barriers of single lasers. Here we propose and demonstrate a novel approach to beam combination and power scaling based on Raman conversion in diamond. Power from multiple non‐collinear pump beams is efficiently transferred onto a single Stokes beam in a single‐pass amplifier. Using three mutually‐independent nanosecond pulsed beams from a free‐running‐linewidth 1064 nm laser, 69% of the total peak pump power of 6.7 kW was transferred onto a TEM₀₀ Stokes seed pulse at 1240 nm in a 9.5 mm long diamond crystal. Compared to other beam combination techniques, diamond beam combination has advantages of relaxed constraints on pump beam mutual coherence, while enabling narrowband output. Thermal considerations for extending from low duty‐cycle to continuous wave operation and higher power levels are discussed.

     

Control of surface charge for high‐fidelity nanostructuring of materials

The universal problem of surface charging during focused ion milling has been fully resolved using a flood‐gun approach based on simultaneous co‐illumination with a UV light‐emitting diode (LED). Non‐distorted as‐designed nano‐patterns were milled using Ga⁺ ions on dielectric materials which charge up strongly. Deep‐UV (250–280 nm) LED co‐illumination during the ion beam milling fully discharges optically the surface under standard Ga⁺ ion‐milling conditions. Photo‐ionization of electrons trapped at the sub‐surface defects to the free vacuum state is a key to the phenomenon ( nm corresponds to a photon energy  eV). The method is applicable as a solution to other charging problems where electrons (primary or secondary) and their spatial redistribution affect nanofabrication or imaging.     

Three‐dimensional ultra‐broadband integrated tapered mode multiplexers

The demonstration of a three‐dimensional tapered mode‐selective coupler in a photonic chip is reported. This waveguide‐based, ultra‐broadband mode multiplexer was fabricated using the femtosecond laser direct‐write technique in a boro‐aluminosilicate glass chip. A three‐core coupler has been shown to enable the multiplexing of the LP₀₁, LP and LP spatial modes of a multimode waveguide, across an extremely wide bandwidth exceeding 400 nm, with low loss, high mode extinction ratios and negligible mode crosstalk. Linear cascades of such devices on a single photonic chip have the potential to become a definitive technology in the realization of broadband mode‐division multiplexing for increasing optical fiber capacity.     

A broadband,quasi‐continuous,mid‐infrared supercontinuum generated in a chalcogenide glass waveguide

The production of a broadband supercontinuum spanning from 1.8 μm to >7.5 μm is reported which was created by pumping a chalcogenide glass waveguide with ≈320 fs pulses at 4 μm. The total power was ≈20 mW and the source brightness was 100 that of current synchrotrons. This source promises to be an excellent laboratory tool for infrared microspectroscopy.     

Room temperature all‐silicon photonic crystal nanocavity light emitting diode at sub‐bandgap wavelengths

Silicon is now firmly established as a high performance photonic material. Its only weakness is the lack of a native electrically driven light emitter that operates CW at room temperature, exhibits a narrow linewidth in the technologically important 1300–1600 nm wavelength window, is small and operates with low power consumption. Here, an electrically pumped all‐silicon nano light source around 1300–1600 nm range is demonstrated at room temperature. Using hydrogen plasma treatment, nano‐scale optically active defects are introduced into silicon, which then feed the photonic crystal nanocavity to enhance the electrically driven emission in a device via Purcell effect. A narrow ( nm) emission line at 1515 nm wavelength with a power density of is observed, which represents the highest spectral power density ever reported from any silicon emitter. A number of possible improvements are also discussed, that make this scheme a very promising light source for optical interconnects and other important silicon photonics applications.     

Efficient Raman frequency conversion of high‐power fiber lasers in diamond

We report high‐power frequency conversion of a Yb‐doped fiber laser using a double‐pass pumped external‐cavity diamond Raman oscillator. Pumping with circular polarization is shown to be efficient while facilitating high‐power optical isolation between the pump and Raman laser. We achieved continuous‐wave average power of 154 W with a conversion efficiency of 50.5% limited by backward‐amplified light in the fiber laser. In order to prove further scalability, we achieved a maximum steady‐state Raman‐shifted output of 381 W with 61% conversion efficiency and excellent beam quality using 10 ms pump pulses, approximately a thousand times longer than the transient thermal time‐constant. No power saturation or degradation in beam quality is observed. The results challenge the present understanding of heat deposition in Raman crystals and foreshadow prospects for reduced thermal effects in diamond than originally anticipated. We also report the first experimental evidence for stimulated Brillouin scattering in diamond.

     

Fiber‐based light sources for biomedical applications of coherent anti‐Stokes Raman scattering microscopy

During the past decade coherent anti‐Stokes Raman scattering (CARS) microscopy has evolved to one of the most powerful imaging techniques in the biomedical sciences, enabling the label‐free visualization of the chemical composition of tissue in vivo in real time. While the acquisition of high‐contrast images of single cells up to large tissue sections enables a wide range of medical applications from routine diagnostics to surgical guidance, to date CARS imaging is employed in fundamental research only, essentially because the synchronized multiple wavelength pulsed laser sources required for CARS microscopy are large, expensive and require regular maintenance. Laser sources based on optical fibers can overcome these limitations combining highest efficiency and peak powers with an excellent spatial beam profile and thermal stability. In this review we summarize the different fiber‐based approaches for laser sources dedicated to coherent Raman imaging, in particular active fiber technology and passive fiber‐based frequency conversion processes, i.e. supercontinuum generation, soliton self‐frequency shift and four‐wave mixing. We re‐evaluate the ideal laser parameters for CARS imaging and discuss the suitability of different laser concepts for turn‐key operation required for routine application in clinics.

     

Mapping the near fields of plasmonic nanoantennas by scattering‐type scanning near‐field optical microscopy

Near‐field optical microscopy techniques provide information on the amplitude and phase of local fields in samples of interest in nanooptics. However, the information on the near field is typically obtained by converting it into propagating far fields where the signal is detected. This is the case, for instance, in polarization‐resolved scattering‐type scanning near‐field optical microscopy (s‐SNOM), where a sharp dielectric tip scatters the local near field off the antenna to the far field. Up to now, basic models have interpreted S‐ and P‐polarized maps obtained in s‐SNOM as directly proportional to the in‐plane ( or ) and out‐of‐plane () near‐field components of the antenna, respectively, at the position of the probing tip. Here, a novel model that includes the multiple‐scattering process of the probing tip and the nanoantenna is developed, with use of the reciprocity theorem of electromagnetism. This novel theoretical framework provides new insights into the interpretation of s‐SNOM near‐field maps: the model reveals that the fields detected by polarization‐resolved interferometric s‐SNOM do not correlate with a single component of the local near field, but rather with a complex combination of the different local near‐field components at each point (, and ). Furthermore, depending on the detection scheme (S‐ or P‐polarization), a different scaling of the scattered fields as a function of the local near‐field enhancement is obtained. The theoretical findings are corroborated by s‐SNOM experiments which map the near field of linear and gap plasmonic antennas. This new interpretation of nanoantenna s‐SNOM maps as a complex‐valued combination of vectorial local near fields is crucial to correctly understand scattering‐type near‐field microscopy measurements as well as to interpret the signals obtained in field‐enhanced spectroscopy.

     

Microresonator Kerr frequency combs with high conversion efficiency

Microresonator‐based Kerr frequency comb (microcomb) generation can potentially revolutionize a variety of applications ranging from telecommunications to optical frequency synthesis. However, phase‐locked microcombs have generally had low conversion efficiency limited to a few percent. Here we report experimental results that achieve conversion efficiency ( on‐chip comb power excluding the pump) in the fiber telecommunication band with broadband mode‐locked dark‐pulse combs. We present a general analysis on the efficiency which is applicable to any phase‐locked microcomb state. The effective coupling condition for the pump as well as the duty cycle of localized time‐domain structures play a key role in determining the conversion efficiency. Our observation of high efficiency comb states is relevant for applications such as optical communications which require high power per comb line.

     

Generation of sub‐terahertz repetition rates from a monolithic self‐mode‐locked laser coupled with an external Fabry‐Perot cavity

A novel scheme to multiply the repetition rate of a monolithic self‐mode‐locked laser for generating sub‐terahertz pulse sources is successfully demonstrated. A coated Yb:KGW crystal is designed to achieve a self‐mode‐locked operation at a repetition rate of 24 GHz with an average output power exceeding 1.0 W at a pump power of 4.8 W. A partially reflective mirror is utilized to combine with the output surface of the gain medium to constitute an external Fabry‐Perot cavity. It is theoretically and experimentally verified that adjusting the external cavity length to satisfy the commensurate condition can lead to the frequency spacing to be various order harmonics of the mode spacing of the monolithic cavity. The maximum pulse repetition rate of the laser output can be up to 216 GHz and the pulse duration is as short as 330 fs. More importantly, the overall characteristics of the first‐order temporal autocorrelation traces obtained by sequentially scanning the external cavity.length display an intriguing phenomenon of temporally fractional revivals, similar to the feature of spatial Talbot revivals.

     

Eye‐safe UV stand‐off Raman spectroscopy for the ranged detection of explosives in the field

Increasing worldwide terrorist attacks involving explosives presents a growing need for a rapid and ranged explosive detection method that can safely be deployed in the field. Stand‐off Raman spectroscopy shows great promise; however, the radiant exposures of lasers required for adequate signal generation are often much greater than what is safe for the eye or the skin, restricting use of the technique to unpopulated areas. Here, by determining the safe exposure levels for lasers typically used in Raman spectroscopy, optimal parameter values are identified, which produce the largest possible detection range using power densities that do not exceed the eye‐safe limit. It is shown that safe ultraviolet pulse energies can be more than three orders of magnitude greater than equivalent safe visible pulse energies. Coupling this to the 16‐fold increase in Raman signal obtained in the ultraviolet at 266 nm over that at 532 nm results in a 131 times larger detection range for the eye‐safe 266‐nm system over an equivalent eye‐safe 532‐nm laser system. For the Raman system described here, this translates to a maximum range of 42 m for detecting Teflon with a 266‐nm laser emitting a 100‐mm diameter beam of 23.5‐mJ nanosecond pulses. Copyright © 2015 John Wiley & Sons, Ltd.     

Beryllium Silicate,Be2SiO4 (phenakite) – a Novel Trigonal SRS‐Active Crystal

In single crystals of the beryllium silicate Be₂SiO₄ with trigonal symmetry , known also as the mineral phenakite, χ⁽³⁾‐nonlinear lasing by stimulated Raman scattering (SRS) is investigated. All observed Stokes and anti‐Stokes lasing components are identified and ascribed to a single SRS‐promoting vibration mode with ω_SRS ≈876 cm⁻¹. With picosecond single‐wavelength pumping at one micrometer the generation of an octave‐spanning Stokes and anti‐Stokes comb is observed.     

Nonlinear absorption and refraction in crystalline silicon in the mid‐infrared

The wavelength dependence of the nonlinear absorption and the third order nonlinear refraction of crystalline silicon between m and m as well as at m have been measured. It was found that at all wavelengths multi‐photon and free carrier absorption can be significant. In particular nonlinear absorption can affect silicon devices designed for the mid‐infrared that require strong nonlinear response, such as for the generation of a supercontinuum.     

The generation of amplified spontaneous emission in high‐power CPA laser systems

An analytical model is presented describing the temporal intensity contrast determined by amplified spontaneous emission in high‐intensity laser systems which are based on the principle of chirped pulse amplification. The model describes both the generation and the amplification of the amplified spontaneous emission for each type of laser amplifier. This model is applied to different solid state laser materials which can support the amplification of pulse durations . The results are compared to intensity and fluence thresholds, e.g. determined by damage thresholds of a certain target material to be used in high‐intensity applications. This allows determining if additional means for contrast improvement, e.g. plasma mirrors, are required for a certain type of laser system and application. Using this model, the requirements for an optimized high‐contrast front‐end design are derived regarding the necessary contrast improvement and the amplified “clean” output energy for a desired focussed peak intensity. Finally, the model is compared to measurements at three different high‐intensity laser systems based on Ti:Sapphire and Yb:glass. These measurements show an excellent agreement with the model.

     

Spectral engineering of coupled open‐access microcavities

Open‐access microcavities are emerging as a new approach to confine and engineer light at mode volumes down to the λ³ regime. They offer direct access to a highly confined electromagnetic field while maintaining tunability of the system and flexibility for coupling to a range of matter systems. This article presents a study of coupled cavities, for which the substrates are produced using Focused Ion Beam milling. Based on experimental and theoretical investigation the engineering of the coupling between two microcavities with radius of curvature of 6 m is demonstrated. Details are provided by studying the evolution of spectral, spatial and polarisation properties through the transition from isolated to coupled cavities. Normal mode splittings up to 20 meV are observed for total mode volumes around . This work is of importance for future development of lab‐on‐a‐chip sensors and photonic open‐access devices ranging from polariton systems to quantum simulators.

     

Mid‐infrared supercontinuum covering 2.0–16 μm in a low‐loss telluride single‐mode fiber

A mid‐infrared (MIR) supercontinuum (SC) has been demonstrated in a low‐loss telluride glass fiber. The double‐cladding fiber, fabricated using a novel extrusion method, exhibits excellent transmission at 8–14 μm: < 10 dB/m in the range of 8–13.5 μm and 6 dB/m at 11 μm. Launched intense ultrashort pulsed with a central wavelength of 7 μm, the step‐index fiber generates a MIR SC spanning from ∼2.0 μm to 16 μm, for a 40‐dB spectral flatness. This is a fresh experimental demonstration to reveal that telluride glass fiber can emit across the all MIR molecular fingerprint region, which is of key importance for applications such as diagnostics, gas sensing, and greenhouse CO₂ detection.

     

Lasing of Nd3+ in sapphire

We present a rare‐earth‐doped sapphire laser. Single‐crystalline α‐Al₂O₃ films doped with trivalent neodymium have been grown by pulsed laser deposition on undoped sapphire substrates. The Nd³⁺ doping concentrations of the films have been varied between 0.3 at.% and 2 at.%. Epitaxial growth was proven by structural and optical characterization of the films. The samples exhibit strongly polarization dependent emission transitions from the ⁴F_3/2 manifold with a fluorescence lifetime of 108 μs and peak emission cross sections of 1.1 × 10⁻¹⁸ cm² around 1100 nm. Lasing at 1096.5 nm was achieved under Ti:sapphire‐pumping in a planar waveguide configuration with a maximum cw output power of 137 mW and a slope efficiency of 7.5% with respect to the incident pump power.

     

Super‐resolution deep imaging with hollow Bessel beam STED microscopy

Stimulated emission depletion (STED) microscopy has become a powerful imaging and localized excitation method, breaking the diffraction barrier for improved spatial resolution in cellular imaging, lithography, etc. Because of specimen‐induced aberrations and scattering distortion, it is a great challenge for STED to maintain consistent lateral resolution deep inside specimens. Here we report on deep imaging STED microscopy using a Gaussian beam for excitation and a hollow Bessel beam for depletion (GB‐STED). The proposed scheme shows an improved imaging depth of up to about 155 μm in a solid agarose sample, 115 μm in polydimethylsiloxane, and 100 μm in a phantom of gray matter in brain tissue with consistent super resolution, while standard STED microscopy shows a significantly reduced lateral resolution at the same imaging depth. The results indicate the excellent imaging penetration capability of GB‐STED, paving the way for deep tissue super‐resolution imaging and three‐dimensional precise laser fabrication.

     

PT symmetry in a fractional Schrödinger equation

We investigate the fractional Schrödinger equation with a periodic ‐symmetric potential. In the inverse space, the problem transfers into a first‐order nonlocal frequency‐delay partial differential equation. We show that at a critical point, the band structure becomes linear and symmetric in the one‐dimensional case, which results in a nondiffracting propagation and conical diffraction of input beams. If only one channel in the periodic potential is excited, adjacent channels become uniformly excited along the propagation direction, which can be used to generate laser beams of high power and narrow width. In the two‐dimensional case, there appears conical diffraction that depends on the competition between the fractional Laplacian operator and the ‐symmetric potential. This investigation may find applications in novel on‐chip optical devices.

     

Suppression and restoration of disorder‐induced light localization mediated by ‐symmetry breaking

We uncover that the breaking point of the ‐symmetry in optical waveguide arrays has a dramatic impact on light localization induced by the off‐diagonal disorder. Specifically, when the gain/loss control parameter approaches a critical value at which ‐symmetry breaking occurs, a fast growth of the coupling between neighboring waveguides causes diffraction to dominate to an extent that light localization is strongly suppressed and the statistically averaged width of the output pattern substantially increases. Beyond the symmetry‐breaking point localization is gradually restored, although in this regime the power of localized modes grows upon propagation. The strength of localization monotonically increases with disorder at both broken and unbroken ‐symmetry. Our findings are supported by statistical analysis of parameters of stationary eigenmodes of disordered‐symmetric waveguide arrays and by analysis of dynamical evolution of single‐site excitations in such structures.