Properties of the 3/2−[521] band in the odd-N rare-earth nuclei

High-spin states in ¹⁶¹Er have been studied experimentally via the ¹⁵⁰Nd(¹⁶O, 5n) reaction at a beam energy of 86 MeV. Three rotational bands built on the 5/2⁺[642], 3/2⁻[521], and 11/2⁻[505] configurations have been extended up to high-spin states, and particularly, the α = −1/2 branch of the ground state 3/2⁻[521] band has been revised significantly. It is found that signature inversion occurs in the 3/2⁻[521] band after the band crossing in ¹⁶¹Er. The systematics of the signature inversion associated with the 3/2⁻[521] configuration in the rare-earth region is discussed. The band properties are analyzed within the framework of a triaxial particle-rotor model, and a triaxial deformation is proposed to the 3/2⁻[521] band.

     

Inelastic excitation of <Superscript>187</Superscript>Re

Excited states in ¹⁸⁷Re populated by inelastic scattering of a 500 MeV ⁸²Se beam have been studied by means of in-beam γ-ray spectroscopy. Levels built on the 5/2⁺[402] and 9/2^-[514] one-quasiparticle states were measured up to I ^π = (21/2⁺) and (21/2^-), respectively. In addition, several new levels including an isomer at 1682 keV with a half-life of 114(23) ns have been found. Quasiparticle configurations of the levels and the transition rates are discussed. Received: 12 December 2002 / Accepted: 13 March 2003 / Published online: 13 May 2003     

Rotational bands in 181Ta

High-spin states in ¹⁸¹Ta have been studied via the ¹⁷⁶Yb(¹¹B,α2n) reaction at 52 MeV using the PEX array and at 57 MeV using the NORDBALL array, with α-particle detection. The previously known, K^π=(7/2)⁺ ground state band and K^π=(9/2)⁻ band have been extended to spins (29/2)⁺ and (31/2)⁻, respectively. Two new one-quasiparticle bands, the K^π=(5/2)⁺ band built on the known (5/2)⁺ isomer and a K^π=((1/2)⁻) band have been observed. Two other rotational bands with three-quasiparticle structure, K^π=(15/2)⁻ and ((19/2)⁺ with π(7/2)[404]ν²(1/2)[510](9/2)[624] and π(9/2)[514]ν²(1/2)[510](9/2)[624] configurations, respectively, have been newly observed. The half-life of the K^π=((19/2)⁺) bandhead which decays to the head of the (15/2)⁻ band has been measured to be 140(36) ns. However, transitions from the ((19/2)⁺) state to the (15/2)⁻ band have not been observed. Received: 26 August 1998     

Experimental Study of High-Spin States in Deformed Odd-Odd 180 Ir

High spin states in deformed odd-odd ¹⁸⁰Ir have been investigated using the ¹⁵⁴Sm (³¹P, 5nγ)¹⁸⁰Ir reaction through the measurements of excitation functions at 150, 155, 160, 165 and 170 MeV beam energies, K X-γ and γ-γ coincidences at 160 MeV. A new level scheme composed of 5 rotational bands has been established. According to the band structure characteristics and the deduced in band B(M1)/B(E2) ratios, the quasiparticle configurations and spin and parity have been proposed to the observed bands. The neutron AB crossing is observed at hω_c≈0.26 MeV for the π1/2^－[541]⊙ν1/2^－[521] and π1/2^－[541]⊙ν5/2^－[512] bands. This AB crossing frequency is close to that in the ν5/2^－[512] band of ¹⁷⁹Os indicating the loss of intruder nature of the π1/2 - orbit. Gradual alignment gain in both the π9/2^－[514]⊙ν7/2⁺[633] and π9/2^－ν5/2^－[512] bands is observed which is similar to the low spin anomaly in alignment in the πh_11/2,πd_5/2 and πi_13/2 bands of neighboring Ir and Re isotopes. Different alignment properties have been discussed in the framework of cranked shell model, and a larger quadrupole deformation is suggested for the bands with π9/2^－[514] orbit involved.     

Laser spectroscopy of the B[17.7]8-X8 and C[19.3]9-X8 transitions of holmium monochloride

Several new transitions of holmium monochloride (HoCl) have been studied at high resolution using laser excitation spectroscopy. Two main transitions, B[17.7]8-X8 and C[19.3]9-X8 have been observed and five bands, 0-0, 0-1, 1-0, 1-1, and 2-1 of the B-X transition and three bands, 0-0, 0-1, and 0-3 of the C-X transition have been obtained at high resolution and rotationally analyzed. Among several low lying states observed in dispersed fluorescence was a strong transition from the C state to a state ∼2140 cm⁻¹ above the ground state. Excitation spectra of this transition have shown that there are apparently two states, ∼6 cm⁻¹ apart. Comparison with ligand field theory calculations are consistent with assigning these states to the excited low lying Ho⁺(4f¹¹6s)Cl⁻ configuration. Several other low lying electronic states have been observed in dispersed fluorescence spectra. Although their assignments could not be established, their energies suggest that they are from the Ho⁺(4f¹⁰6s²)Cl⁻ or Ho⁺(4f¹¹6s)Cl⁻ configurations. Rotational constants have been obtained for the B[17.7]8 and C[19.3]9 states and have been used to speculate on the possible electron configurations for these states.     

Nuclear levels in 238Np

Low and high energy spectra from thermal neutron capture in ²³⁷Np have been studied over the energy ranges 25 to 650 keV and 2600 to 5500 keV. Primary transitions from neutron capture in four resonances have been observed between about 4800 and 5400 keV. Using 12 MeV deuterons, (d, p) spectra at three angles have been observed with a magnetic spectrograph. A nuclear level scheme for ²³⁸Np has been constructed by combining the results of the above measurements with previous data from a study of the ^242mAm α-decay. The Nilsson model has been used to interpret the level structure. Including results from the previous α-decay study, nine rotational bands can be assigned. The Nilsson configurations (K^π [Nn₃ΛΣ]) and band-head energies are: 2⁺π[642↑]?ν[631↓], 0.0 keV; 3⁺π[642↑]+ν[631↓], 86.6 keV; 3^?π[523↓]+ν[631↓], 136.0 keV; 2^?π[523↓]?ν[631↓], 182.8 keV; 5⁺π[642↑]+ν[622↑], 278.1 keV; 0⁺π[642↑]?ν[622↑], 332.5 keV; 5^?π[523↓]+ν[622↑], 342.6 keV; 0^?π[523↓]?ν[622↑], 286.0 keV; 6^?π[642↑]+ν[743↑], 301 keV. The measured (d, p) reaction cross sections are compared with theoretical calculations based on these assignments. The Gallagher-Moszkowski rule is found to be valid in the four cases where we have observed both parallel and antiparallel coupled bands with $\text{K}{}^{\mathrm{+}}\text{= Ω}{}_{\mathrm{<mtext>p</mtext>}}\text{+Ω}{}_{\mathrm{<mtext>n</mtext>}}$ and $\text{K}{}^{\mathrm{?}}\text{= |Ω}{}_{\mathrm{<mtext>p</mtext>}}\text{?Ω}{}_{\mathrm{<mtext>p</mtext>}}\text{|}$. The lowest levels of the two K = 0 bands have spin I = 1; Newby odd-even shifts can be determined in both cases.     

Structure analysis of 159Sm and properties of odd-mass neutron-rich nuclei in mass-160 region

Recent fission experiment data provide interesting structure information for neutron-rich nuclei in the mass A ∼ 160 region. We apply the projected shell model to study the strongly-deformed, neutron-rich Sm isotopes. We perform calculations for rotational bands up to spin I = 20 (29/2) for even-even (odd-neutron) Sm isotopes, and analyze the band structure of low-lying states with quasiparticle excitations. Emphasis is given to rotational bands based on one-quasiparticle (1-qp) configurations in the odd-mass ¹⁵⁹Sm. The ¹⁵⁹Sm result is discussed together with those of the even-even isotopes ^158,160Sm. New bands in ¹⁵⁹Sm based on neutron 1-qp 1/2⁻ and 5/2⁺ configurations are predicted. Electromagnetic transition probabilities are discussed.

     

Study of low-lying states in151Eu via (n,n′γ) reaction

The levels of¹⁵¹Eu have been investigated in the (n,n′γ) reaction using nuclear reactor fast neutrons. The energies, intensities and angular distributions of theγ-rays have been measured with the Ge(Li) spectrometer. Four rotational bands with the following band heads and Nilsson configurations have been identified: ground state band, 5/2⁺ [402]; 21.5 keV, 7/2⁺[404]; 196.5 keV, 3/2⁺[411]; 260.5 keV, 5/2⁺[413]. The low spin states at 332.2 and 336.2 keV have been tentatively assigned to the l/2⁺[411] Nilsson orbital, but 522.8, 580.0 and 587.0 keV states to the 1/2⁺[420] Nilsson orbital. The negative parity levels at 353.7, 522.1 and probably 546.2 keV have been proposed basing on theh _11/2 proton state.     

SO2: High-resolution analysis of the (0 3 0), (1 0 1), (1 1 1), (0 0 2) and (2 0 1) vibrational states; determination of equilibrium rotational constants for sulfur dioxide and anharmonic vibrational constants

High resolution Fourier transform spectra of a sample of sulfur dioxide, enriched in ³⁴S (95.3%). were completely analyzed leading to a large set of assigned lines. The experimental levels derived from this set of transitions were fit to within their experimental uncertainties using Watson-type Hamiltonians. Precise band centers, rotational and centrifugal distortion constants were determined. The following band centers in cm⁻¹ were obtained: ν₀(3ν₂)=1538.720198(11), ν₀(ν₁ + ν₃)=2475.828004(29), ν₀(ν₁ + ν₂ + ν₃)=2982.118600(20), ν₀(2ν₃)=2679.800919(35), and ν₀(2ν₁ + ν₃)=3598.773915(38). The rotational constants obtained in this work have been fit together with the rotational constants of lower-lying vibrational states [W.J. Lafferty, J.-M. Flaud, R.L. Sams, EL Hadjiabib, J. Mol. Spectrosc. 252 (2008) 72-76] to obtain equilibrium constants as well as vibration-rotation constants. These equilibrium constants have been fit together with those of ³²S¹⁶O₂ [J.-M. Flaud, W.J. Lafferty, J. Mol. Spectrosc. 16 (1993) 396-402] leading to an improved equilibrium structure. Finally the observed band centers have been fit to obtain anharmonic rotational constants.     

Study of Collective Rotational Bands in 179Pt

High-spin states in ¹⁷⁹Pt have been studied experimentally using the ¹⁴⁹Sm(³⁵Cl, p4n) fusion-evaporation reaction at beam energies of 164—180MeV. Measurements of γ-ray excitation function, X-γ coincidences and γ-γ-t coincidences were carried out with 13 BGO(AC) HPGe and 3 LOAX detectors. Based on the measured results, three rotational bands built on intrinsic states assigned to the 1/2^－[521], 5/2^－[512] and 7/2⁺[633] Nilsson configurations have been established for ¹⁷⁹Pt. It has been observed that the aligned angular moment in the 1/2^－[521] band increases suddenly around hω=0.27MeV. The big signature splitting has been observed in the 7/2⁺[633] band. These phenomena are discussed by referring to the systematics of the level structure in the Pt isotopes and isotones of ¹⁷⁹Pt.     

g-factor measurement of the two lowest 10+ states in 140Sm

The g-factors of the two 10⁺ states in ¹⁴⁰Sm at 3172 and 3210 keV have been measured by means of the TDPAD method. The obtained values are g = −0.176(20) and g = 1.27(9), respectively. The reaction ¹¹⁶Cd (²⁸Si, 4n)¹⁴⁰Sm, at incident beam energy of 125 MeV, has been used. The measured values clearly show that these states can be described as rather pure (νh_11/2)⁻² and (πh_11/2)² configurations.     

T-band phenomena in 183Re

Abstact: High-spin states in ¹⁸³Re have been studied using the ¹⁷⁶Yb(¹¹B,4n) reaction at 52 and 57 MeV. Two high-K bands have been observed directly by a time-correlated γ-γ coincidence measurement. One of the bands is built on an isomeric K ^π=(25/2)⁺ state at E _x= 1908 keV with a half-life of 0.82(2) ms. The other band, assigned as K ^π=(29/2)⁻ at E _x= 2739 keV, decays to the (25/2)⁺ band. These bands are interpreted as three-quasiparticle structures, π(5/2)⁺[402] &⊗ν(9/2)⁺[624] ⊗ν(11/2)⁺[615] for the (25/2)⁺ band and π(9/2)⁻[514] ⊗ν(9/2)⁺[624] ⊗ν(11/2)⁺[615] for the (29/2)⁻ band. The K ^π= (29/2)⁻ band becomes strongly Coriolis mixed with increasing spin and is gradually changing into a low-K s-band structure. Received: 20 April 1998     

Backbendings of superdeformed bands in ~(36,40)Ar

Experimentally observed superdeformed(SD) rotational bands in ~(36)Ar and ~(40)Ar are studied by the cranked shell model(CSM) with the pairing correlations treated by a particle-number-conserving(PNC) method.This is the first time that PNC-CSM calculations have been performed on the light nuclear mass region around A=40.The experimental kinematic moments of inertia J~((1))versus rotational frequency are reproduced well. The backbending of the SD band at frequency around ω =1.5 Me V in ~(36)Ar is attributed to the sharp rise of the simultaneous alignments of the neutron and proton 1 d_(5/2)[202]5/2 pairs and 1 f_(7/2)[321]3/2 pairs, which is a consequence of the band crossing between the 1 d_(5/2)[202]5/2 and 1 f_(7/2)[321]3/2 configuration states. The gentle upbending at low frequency of the SD band in ~(40)Ar is mainly affected by the alignments of the neutron 1 f_(7/2)[321]3/2 pairs and proton 1 d_(5/2)[202]5/2 pairs.The PNC-CSM calculations show that besides the diagonal parts, the off-diagonal parts of the alignments play an important role in the rotational behavior of the SD bands.     

Investigation into the rotational bands of 185Pt with the particle-rotor model

Theoretical calculations have been performed for the ν9/2⁺[624](i _13/2) and ν7/2⁻[503]( f _7/2) bands of ¹⁸⁵Pt in the framework of particle-rotor model. The band properties of signature splitting and configuration mixing have been analyzed. The level energy and signature splitting before the band crossing can be well interpreted by introducing triaxiality. The positive-parity yrast band is proposed to be dominated by the ν9/2⁺[624](i _13/2) component, while the negative-parity band shows strong mixing of ν7/2⁻[503](f _7/2) and ν9/2⁻[505](h _9/2) configurations.

     

Structure of the doubly odd nucleus 180Ta: Description of 23 bands

The structure of the doubly-odd nucleus ¹⁸⁰Ta has been studied by γ–γ coincidence measurements with a DC beam at 52 and 57 MeV and time-correlated γ–γ coincidence measurements with a pulsed beam at 55 MeV via the ¹⁷⁶Yb(¹¹B, α3n)¹⁸⁰Ta reaction. In all measurements, γ-rays were detected in coincidence with charged particles. In the time-correlated γ–γ coincidence measurements with a pulsed ¹¹B beam, three rotational bands and one octupole vibrational band have been identified above the I^π=15⁻ T_1/2=30 μs isomer. The configuration of three bands built on 8⁺ states has been discussed by means of three-band mixing calculations. BCS calculations with blocking have been used in support of configuration assignment of four- and six-quasiparticle structures. Totally, 19 rotational bands, one β-, one γ- and two octupole-vibrational bands, plus one intrinsic state have been identified with two-, four- and six-quasiparticle configurations. The K values of these bands range from 0 to 19. The K-forbidden transition rates are discussed on the basis of mixing between states with widely different K-values. The BBCS calculations predict a K^π=22⁻ isomer not identified experimentally in this nor in previous works.A search for specific intermediate states which could explain the transformation from K^π=9⁻ to 1⁺ during the astrophysical s- and r- processes was negative.     

New rotational bands in 174Ta

Three new bands in ¹⁷⁴Ta have been identified by using the ¹⁶⁰Gd(¹⁹F,5n) reaction at beam energies of 87 MeV and 96 MeV. Nilsson configurations are assigned to these bands. In the 9/2⁻[514]_p+5/2⁻[512]_n band, the AB neutron crossing occurs at a rotational frequency of 0.30 MeV. This is indicative of the disappearance of the evidence for a reduction in neutron pair correlations. Received: 30 March 1998     

Isomeric state at 945.3 keV in237Np

A new isomeric state in²³⁷Np has been discovered at an excitation energy of (945.3±0.2) keV withT _1/2 =(711±40) ns. Six gamma-ray lines have been measured depopulating the isomeric state to known levels in²³⁷Np. The comparison of the measured absolute gamma-ray transition probabilities with empirical values yields as most probable spinI andK assignmentI=K=13/2 for this isomeric state. It is most likely a 1-proton-2-neutron quasiparticle state 13/2^?π5/2⁺ [642] +ν7/2^? [743] + ν 1/2⁺ [631]. However, a one-quasiparticle 11/2^? [505] configuration for the isomer cannot be excluded.     

Analysis of the ν9 and ν10 bands of cyclopropane

The infrared spectrum of gaseous cyclopropane has been measured in the regions 980–1080 and 1400–1500 cm^?1, containing the ν₁₀ and ν₉E′ fundamental bands, respectively, using a high-resolution Fourier transform instrument. Deconvolution was used to enhance the resolution in the crowded parts of the spectrum to ～0.0020–0.0025 cm^?1. Apart from the rotational l-resonance affecting mainly the low-K subbands, the ν₉ band is strongly perturbed by Fermi resonance with the 2ν₁₄² state lying ～41 cm^?1 above. The effects of the Fermi resonance are most pronounced in the high-KΔK = +1 subbands as the 2ν₁₄^?2 levels would cross the ν₉⁺ levels near K = 30. ^rR lines of 2ν₁₄^?2 for K = 24 to 36, enhanced by the resonance, have been identified in the region 1469–1475 cm^?1 of the spectrum. Two extra perturbation-enhanced subbands are found adjacent to the K = 16?17 and K = 17?16 subbands of ν₉: these have been ascribed to the K = 18?17 transitions in 2ν₁₄^?2 and to the K = 19?16 transitions in $\text{ν}{}_2\text{2ν}{}_{14}{}^0$, respectively, as their upper states coincide with the corresponding levels ν₉^?(K = 16) and ν₉⁺(K = 17). A combination of l-resonance and Fermi resonance is mainly responsible for the interactions causing the perturbations and appearance of the extra subbands, but a direct rotational interaction 〈ν₉^?(K)|h₃|2ν₁₄^?2(K + 2)〉 also had to be introduced to accurately account for the observations. In contrast, the ν₁₀ band is not appreciably perturbed by other states and merely exhibits effects of strong l-resonance in the low-K subbands, and K-doubling of the high-J lines of the K = 2–3 subband. A detailed analysis of the spectrum and of the perturbations is described and sets of accurate spectroscopic constants are reported for ν₁₀ and ν₉ as well as for the perturbing state 2ν₁₄², which reproduce 3020 observed lines of the ν₁₀ band with a standard deviation of 0.0008 cm^?1 and 1810 lines of ν₉ with a standard deviation of 0.0010 cm^?1.     

The methane ν1(a1) vibrational state rotational structure obtained from high-resolution CARS-spectra of the Q-branch

The gaseous methane ν₁(a₁), Q-branch coherent anti-Stokes Raman scattering (CARS) spectra have been investigated at a resolution of 0.002 cm^?1. A complex rotational structure of the resolved Q-branch has been experimentally observed. This structure can be ascribed to strong tetrahedral splitting of the rotational levels of the upper vibrational state, which possibly occurs due to Fermi resonance between the ν₁(a₁) and 2ν₂(a₁) vibrational energy levels which are close to each other. An assignment of the observed spectral lines has been made, yielding the rotational constants B, D, and D_t for the ν₁(a₁) vibrational state of the methane molecule. The absolute Raman frequency ν₁ of the purely vibrational transition has been found.     

The perpendicular band ν14 of benzene near 10 μm

The perpendicular band of the E_1u vibration ν₁₄ of C₆H₆, with band origin at 1038.2670 cm^?1, was measured on a Bomem high-resolution Fourier transform spectrometer with a 246-cm optical path difference. The spectrum was deconvolved to an effective linewidth of ～0.002 cm^?1. A total of 135 subbands have been assigned in the ν₁₄ band. The band was found to be remarkably free of perturbations by other states. A Hamiltonian matrix of order 2, including merely the rotational l-type resonances between the ν₁₄⁺(J, K) and ν₁₄^?(J, K ? 2) levels, was used for the treatment of the upper states of this band. A set of accurate spectroscopic constants was obtained, which reproduces a total of 3258 measured lines with an over-all standard deviation of 0.0006 cm^?1.