Demonstration of long-term reliability of a 266-nm, continuous-wave, frequency-quadrupled solid-state laser using beta-BaB(2)O(4)

We report what we believe to be the first operation of more than 1000 h of a 266-nm (cw) frequency-quadrupled solid-state laser with a 100-mW output. We used beta-BaB(2)O(4)(BBO) crystal grown by the Czochralski method to double the green-light (532-nm) wavelength, using an external resonant cavity. The green light was generated with an intracavity frequency-doubled Nd:YVO(4)laser pumped by a 4-W laser diode. When the incident 532-nm power on the external resonant doubler was 500 mW, we generated 100 mW of cw 266-nm radiation with the BBO crystal. The degradation rate seems to be proportional to the strength of the UV optical electric field. We also obtained a relative intensity noise of -130dB/Hz at frequencies of 2 to 10 MHz for 266-nm laser light.     

Highly efficient infrared-to-visible energy upconversion in Er(3+):Y(2)O(3)

Very intense green and red emission was observed at room temperature from the (4)S(3/2) and (4)F(9/2) levels of Er(3+):Y(2)O(3). A cw diode laser at 975 nm was used as a pump for resonant sequential excitation of the (4)I(11/2) and (4)F(7/2) levels. The fluorescence was easily visible to the naked eye, even with 27 mW of excitation power. It was found that at 850 mW of cw excitation power the total luminance was 39,000 cd/m(2). This corresponds to ~100 muW of green emission and 270 muW of red emission.     

Diode-pumped cw Nd:YAG three-level laser at 869 nm

We report for the first time (to our knowledge) a diode-pumped Nd:YAG laser emitting at 869 nm based on the (4)F(3/2)-(4)I(9/2) transition, generally used for a 946 nm emission. Power of 453 mW at 869 nm has been achieved in cw operation with a fiber-coupled laser diode emitting 35.4 W at 809 nm. Intracavity second-harmonic generation in the cw mode has also been demonstrated with power of 118 mW at 435 nm by using a BiB(3)O(6) nonlinear crystal. In our experiment, we used a LiNbO(3) crystal lens to complement the thermal lens of the laser rod, and we obtained good beam quality and high output power stability.     

Diode-pumped Nd:YAG laser emitting at 899 nm and below

We present what is, to the best of our knowledge, the first diode-pumped Nd:YAG laser emitting at 899 nm and below, based on the (4)F(3/2) - (4)I(9/2) transition, generally used for a 946 nm emission. A power of 630 mW at 899 nm has been achieved in cw operation and 16 mW at 884 nm with a fiber-coupled laser diode emitting 9 W at 808 nm. Intracavity second-harmonic generation in cw mode has also been demonstrated with a power of 100 mW at 450 nm by using a LiB(3)O(5) nonlinear crystal.     

All-solid-state continuous-wave frequency-doubled Nd:YAG-BiBO laser with 2.8-W output power at 473 nm

We report on a diode-pumped Nd:YAG laser with 4.6 W of linear polarized continuous-wave (cw) output power on the 4F3/2 --> 4I9/2 transitions at 946 nm. Three different crystals, cut for critical type I phase matching at room temperature, are used for the intracavity frequency doubling of the laser: 10-mm-long LiBaO5 (LBO), an 8-mm-long beta-BaB2O4 (BBO), and a 10.4-mm-long BiB3O6 (BiBO) grown by FEE GmbH. Up to 2.8 W of cw output power in the blue spectral range at 473 nm has been achieved with the BiBO crystal (2.1 W with BBO and 1.5 W with LBO).     

Affinement d'une raie de fluorescence de Pr3+: LaAlO3 par excitation laser

A cw dye laser has been used for fluorescence line narrowing experiments by resonant excitation on Pr³⁺ ions in LaAlO₃. Scanning the excitation radiation through the absorption line width corresponding to the transition ³H₄ (0 cm^-1) → ¹D₂ (16 694 cm^-1) while fluorescence was observed, has put into evidence a deformation of the symmetry around Pr³⁺ ions, different for every site.This experiment shows the power of cw dye laser spectroscopy for investigating optical spectra in crystals.     

Generation of 740 mW of blue light by intracavity frequency doubling with a first-order quasi-phase-matched KTiOPO(4) crystal

We report on efficient intracavity frequency doubling of a cw diode-pumped Nd:YAG laser on the (4)F(3/2)?(4)I(9/2) laser transition at 946 nm. The nonlinear crystal used in the experiments was a first-order quasi-phase-matched flux-grown KTiOPO(4) crystal (period, 6.09mum ; thickness, 1 mm; length, 9 mm). The fluctuations in the generated second-harmonic wave were lower than 3% at output powers of as much as 500 mW. The overall optical-to-optical efficiency was 5.7%. A maximum output power of 740 mW of blue light was generated, which was stable for only 0.5 min. The decrease the output power at this power level was attributed to heating and thermal lensing in the periodically poled KTiOPO(4) crystal. The short-term behavior of the second-harmonic wave exhibited switching between a cw mode and chaotic intensity fluctuations.     

Continuous-wave solid-state dye laser

We report the first realization of a cw solid-state dye laser. The laser medium consists of a laser dye (Rhodamine 6G) dissolved in a photopolymer. The UV-cured solution is sandwiched between two DVD substrates. The resonator design was derived from a conventional liquid solvent dye laser geometry. The laser radiation can be tuned from 565 to 615 nm by using a birefringent filter. A pump power of 2 W leads to a cw output power of more than 20 mW.     

Efficient power scaling of laser radiation by spectral beam combining

The possibility of achieving multikilowatt laser radiation by spectrally combining beams using volume Bragg gratings (VBGs) is shown. The VBGs recorded in a photothermorefractive glass exhibit long-term stability of all its parameters in high-power laser beams with power density >1 MW/cm2 in the cw beam of total power on a kilowatt level. We consider an architecture-specific beam-combining scheme and address the cross-talk minimization problem based on optimal channel positioning. Five-channel high efficiency spectral beam combining resulted in a >750 W near-diffraction-limited cw beam has been demonstrated experimentally.     

Photoreduction processes and nanocluster formation induced by a CO2 laser on silicate surfaces

The photoreduction processes stimulated either the cw (power density 10⁵–10⁶ W/cm²) or pulsed (pulse energy 3–4 J, pulse duration 200 ns, effective laser spot diameter 1 mm) radiation of a CO₂ laser on the surfaces of fused and crystalline quartz, as well as of natural silicates (nepheline KNa₃[AlSiO₄]₄, rhodonite CaMn₄[Si₅O₁₅], and zircon ZrSiO₄), are studied. The X-ray emission analysis of irradiated surfaces showed that the laser irradiation of these materials leads to the sublimation of silicon oxides and the enrichment of surfaces with constituent metal elements. Laser radiation also stimulates the formation of silicon and metal nanoclusters on irradiated surfaces. The appearance of these nanoclusters is confirmed by both photoluminescence and X-ray emission studies of irradiated surfaces.     

Efficient Nd:Y<Subscript>0.36</Subscript>Gd<Subscript>0.64</Subscript>VO<Subscript>4</Subscript>-GdCa<Subscript>4</Subscript>O(BO<Subscript>3</Subscript>)<Subscript>3</Subscript> red laser under diode pumping into the emitting level

We report a red laser at 671 nm generation by intracavity frequency doubling of a continuous wave (cw) laser operation of a 1342 nm Nd:Y_0.36Gd_0.64VO₄ laser under diode pumping into the emitting level ⁴ F _3/2. An GdCa₄O(BO₃)₃ (GdCOB) crystal, cut for critical type I phase matching at room temperature is used for second harmonic generation of the laser. At an incident pump power of 17.8 W, as high as 1.12 W of cw output power at 671 nm is achieved. The optical-to-optical conversion efficiency is up to 6.3%, and the fluctuation of the red output power was better than 3.5% in the given 30 min.     

Continuous-wave Nd:GdVO<Subscript>4</Subscript>/LBO laser at 541.5 nm under diode pumping into the emitting level

We report a green laser at 541.5 nm generation by intracavity frequency doubling of a continuous wave (cw) laser operation of a 1083 nm Nd:GdVO₄ laser under 880 nm diode pumping into the emitting level ⁴ F _3/2. A LiB₃O₅ (LBO) crystal, cut for critical type I phase matching at room temperature is used for second harmonic generation of the laser. At an incident pump power of 17.8 W, as high as 2.52 W of cw output power at 541.5 nm is achieved. The optical-to-optical conversion efficiency is up to 14.2%, and the fluctuation of the green output power was better than 3.6% in the given 30 min.     

Trace-gas sensor based on mid-IR difference-frequency generation in PPLN with saturated output power

The development and characterization of a compact pulsed mid-IR laser source for sensitive on-line trace-gas analyses in the 3–4 μm wavelength range is reported. The source is based on an advantageous difference-frequency mixing configuration in periodically poled LiNbO₃ (PPLN) with a cw external-cavity diode laser (ECDL; 810–830 nm) for broad and accurate tunability and a diode-pumped passively Q-switched Nd:YAG laser (1064 nm) for high mid-IR peak power. With 5 mW cw pump and 4.7 kW signal peak power incident on a 19 mm long PPLN crystal, a maximum of 360 μW mid-IR peak power was generated. The narrowband (∼150 MHz) radiation was saturated by a factor of 15 compared with the nonsaturated case due to depletion of the pump laser radiation. This results in a very high amplitude stability of the generated mid-IR power and thus in a high detection sensitivity. A minimum detectable absorption coefficient of 2.8×10⁻⁸ cm⁻¹ was achieved in combination with a 36.2 m multipass cell in an averaging time of 20 s, as demonstrated by on-line analyses of formaldehyde traces near 3.53 μm.     

Efficient Nd:Y0.5Gd0.5VO4-KTiOPO4 green laser under diode pumping into the emitting level 4F3/2

We report a green laser at 532 nm generation by intracavity frequency doubling of a continuous wave (cw) laser operation of a 1064 nm Nd:Y_0.5Gd_0.5VO₄ laser under diode pumping into the emitting level ⁴ F _3/2. A KTiOPO₄ (KTP) crystal, cut for critical type-II phase matching at room temperature is used for second harmonic generation (SHG) of the laser. At an incident pump power of 17.8 W, as high as 4.21 W of cw output power at 532 nm is achieved. The optical-to-optical conversion efficiency is up to 23.6%, and the fluctuation of the green output power was better than 2.8% in the given 30 min.     

Diode-pumped singly resonant continuous-wave optical parametric oscillator with wide continuous tuning of the near-infrared idler wave

We demonstrate wide, continuous tuning of the single-frequency idler wave of a cw singly resonant optical parametric oscillator (SRO). The SRO consists of a periodically poled LiNbO(3) crystal for quasi-phase matching in a four-mirror signal-resonant ring cavity. The SRO, excited by 2.25 W of 924-nm radiation from an InGaAs diode laser, generates as much as 200 mW of single-frequency 2.1-mum idler radiation. We tune the idler frequency continuously within a range as large as 56 GHz by changing the wavelength of the diode pump laser. The versatility of this continuously tunable single-frequency infrared source is demonstrated by recording of N(2)O rovibrational absorption lines near 2.1 mum.     

Diode-pumped continuous-wave and femtosecond laser operations of a heterocomposite crystal Yb3+: SrY4(SiO4)3O parallel Y2Al5O12

We report cw and femtosecond laser operations under diode pumping of a diffusion-bonding heterocomposite Yb-doped crystal: Yb3+:SrY4(SiO4)3O parallel Y2Al5O12(YAG paralell SYS:Yb). To show the advantages of this heterocomposite crystal over classical Yb:SYS crystal, we first investigate the high-power cw regime. A cw power of 4.3 W is demonstrated. The femtosecond regime is also investigated, and 1-W-average-power, 130-fs pulses at 1070 nm are produced, which represents, to our knowledge, the first demonstration of an Yb-doped heterocomposite mode-locked laser.     

A continuous wave SrMoO4 Raman laser

We demonstrate a cw, laser diode-pumped Nd:GdVO4/SrMoO4 crystalline Raman laser. First Stokes laser output at 1173.5?nm of 2.18?W was achieved with a diode-to-first Stokes efficiency of 8.7%. With intracavity frequency doubling in LiB3O5, 3.1?W of cw yellow emission at 586.8?nm was obtained with a 12.4% diode-to-yellow efficiency. The experimental results show that SrMoO4 is an excellent stimulated Raman scattering gain material for high-power cw near-IR Stokes and yellow lasers.     

Theory and experiment of CW dye laser injection locking and its application to second harmonic generation

High-power single-mode operation of a cw ring dye laser has been obtained by injection of cw single-mode radiation. The intracavity power of this system was used to generate tunable single-mode uv radiation by frequency doubling in a temperature phase-matched ADA crystal: up to 45 W intracavity fundamental power and up to 70 mW extracted uv power have been observed. A theoretical treatment of the injection locked cw ring dye laser system is given for the stationary state. Expressions for the intracavity intensities as a function of the small-signal gain and the saturation intensity are derived.     

Single-frequency continuous-wave radiation from 0.77 to 1.73 microm generated by a green-pumped optical parametric oscillator with periodically poled LiTaO3

We describe a cw optical parametric oscillator (OPO) with multigrating periodically poled LiTaO(3) . Pumped by a single-frequency 532-nm laser, the OPO emits single-frequency radiation at wavelengths from 0.77 to 1.73mum with as much as 60 mW of output power. Mode-hop-free operation for as long as 50 min, a low frequency drift (<70MHz/h), and as much as 700-MHz continuous frequency tuning of signal and idler are demonstrated.     

Tunable continuous-wave operation of a Cr3+,Li+:Mg2SiO4 laser

Room-temperature tunable cw laser oscillation of Cr3+ ions in forsterite crystals (Mg2SiO4) codoped with chromium and lithium has been demonstrated, for the first time to the authors' knowledge, in pumping a crystal with a Ti:sapphire laser into the first excited level of Cr3+ ions (4A2-4T2 transition). The laser is smoothly tunable in the region of 1095-1170 nm. A slope efficiency as great as 4.4% has been achieved.