Ultrashort-pulse laser irradiation of metal films: the effect of a double-peak laser pulse

The optical properties of blue-violet InGaN light-emitting diodes under normal and reversed polarizations are numerically studied. The best light-emitting performance under normal and reversed polarization is obtained in a single quantum-well structure and double quantum-well structure, respectively. The key factors responsible for these phenomena are presumably the carrier concentration distribution and the amount of carriers in quantum wells. The turn-on voltage of light-emitting diodes under reversed polarization is lower than that of light-emitting diodes under normal polarization, due mainly to lower potential heights for electrons and holes in the active region.     

Wavelength-independent all-optical synchronization of a Q-switched 100-ps microchip laser to a femtosecond laser reference source

We present a Q-switched microchip laser emitting 1064-nm pulses as short as 100 ps synchronized to a cavity dumped femtosecond laser emitting 800-nm pulses as short as 80 fs. The synchronization is achieved by presaturating the saturable absorber of the microchip laser with femtosecond pulses even though both lasers emit at widely separated wavelengths. The mean timing jitter is 40 ps and thus considerably shorter than the pulse duration of the microchip laser.     

Discharge instability induced by external laser preionization of a XeF discharge laser

External-laser-induced preionization of excimer lasers was investigated. A discharge XeF laser was preionized by two different UV lasers [a KrF laser (λ=249 nm) and an ArF laser (λ=193 nm)], and the improvements in performance of the XeF laser were compared. The XeF laser beam profiles were measured by an intensified CCD (ICCD) camera with temporal resolution of 10 ns. Striated XeF laser profiles were obtained with 249 nm laser preionization, whereas there was no striation in the profiles for 193 nm laser preionization. These striations originated from discharge in the XeF laser induced by laser preionization. The influence of excited rare-gas atoms on the discharge instability was examined.     

High-efficiency 2 kW XeCl excimer laser

Received: 15 May 1998 / Revised version: 5 August 1998 / Published online: 24 February 1999     

Experimental implementation of ultrashort laser pulses in the von Neumann picture

The characterization and interpretation of ultrashort laser pulses is most intuitive in the joint time–frequency domain, where structures like multiple pulses become immediately apparent. For practical reasons, ultrafast femtosecond laser pulse shaping, however, is commonly carried out in the frequency domain. Here we implement pulse shaping of optical fields defined in the von Neumann representation, which is a joint time–frequency distribution with complex-valued Gaussian basis functions. We discuss the feasibility as well as the principal limitations of this technique, show illustrative examples, and propose possible applications in coherent control.     

Top-hat cw laser induced thermal mirror: a complete model for material characterization

A complete theoretical model is presented for the thermal mirror technique under top-hat laser excitation. Considering the attenuation of the top-hat excitation laser intensity along the thickness of a sample due to its optical absorption coefficient, we calculate the laser-induced temperature and surface deformation profiles. A simplified theoretical model for a high absorption sample is also developed. The center intensity of a probe beam reflected from the thermal mirror at a detector plane is derived. Numerical simulation shows that the thermal mirror under the top-hat laser excitation is as sensitive as that under Gaussian laser excitation. With top-hat laser excitation, the experimental results of thermo-physical properties of opaque samples are found to be well consistent with literature values, validating the theory.     

Double-pulse LIBS of gadolinium oxide ablated by femto- and nano-second laser pulses

Emission characteristics of gadolinium (Gd) oxide are studied, using ns and fs laser pulses for ablation in double-pulse laser induced breakdown spectroscopy (LIBS). In the current conditions of pulse energy and signal detection timing, emission intensity enhancement in the reheating mode is 25-fold, but little effect can be observed in a pre-pulse mode. It is shown that the optimum focus position of the ablation pulse is about 5 mm apart from the sample surface in the reheating mode. Although little emission can be observed in the single-pulse configuration with fs ablation pulses, the intense emission can be observed in the reheating mode in the double-pulse configuration.     

Photoinduced multiple microchannels inside silicon produced by a femtosecond laser

Photoinduced multiple microchannels in the interior of silicon produced by an 800-nm femtosecond laser were observed. The multiple microchannels were aligned spontaneously with a period along the propagation direction of the laser beam, which could be attributed to the interface spherical aberration induced due to refractive-index mismatch. We also observed that the depth of the photoinduced microchannels increased with the increase of the laser power. The power dependence of the depth of photoinduced microchannels in silicon was different from that in transparent materials, which probably arose from the competition between self-focusing due to the nonlinear Kerr effect and self-defocusing related to the thermal accumulation in the process of laser irradiation.     

High-efficiency direct-pumped Nd:YLF laser operating at 1321 nm

We present a high-efficiency Nd: LiYF₄ (Nd:YLF) laser operating at 1321 nm pumped directly into the emitting level, ⁴F_3/2. The linear polarization of the pump diode laser was maintained by a short fiber. At the absorbed pump power of 7.3 W, as high as 3.6 W of continuous-wave output power at 1321 nm is achieved. The slope efficiency with respect to the absorbed pump power was 0.52. To the best of our knowledge, this is the first demonstration of such a laser system. Comparative results obtained for the pump with a diode laser at 806 nm, into the highly absorbing ⁴F_5/2 level, are given in order to prove the advantages of 880 nm wavelength pumping.     

Determination of the effective upper laser level lifetime from an end-pumped Tm,Ho:YLF laser

We report the measurement of the effective upper laser level lifetime from an end-pumped Q-switched Tm,Ho:YLF laser. When the pump power is 1.58 W, the effective upper laser level lifetime is only 2.5 ms, which is less than the fluorescence lifetime (∼16 ms) of the upper laser level. The dependences of the effective upper laser level lifetime on the pump power and the temperature of laser crystal are firstly obtained experimentally. The experimental results show that the effective upper laser level lifetime decreases with increasing the pump power and the temperature of laser crystal, respectively. Furthermore, the experimental results are compared with the theoretical results.     

Random fiber laser operating at 1,115 nm

We experimentally demonstrate a random fiber laser operating at 1,115 nm using a LD-pumped Yb-doped fiber laser as the pump source. We achieve about 270 mW lasing output in a 50 km standard communication optical fiber with slope efficiency more than 28 %. A new wavelength is provided for the application of random distributed feedback fiber lasers as light sources.     

Modeling of laser induced breakdown spectroscopy for very low-pressure conditions

Laser Induced Breakdown Spectroscopy (LIBS) can be considered as a prominent technology for compositional analysis of materials in low-pressure space applications. In space applications, usually LIBS is conducted in a low-pressure environment and proper understanding of the plasma parameters is significant for any improvement in the system. A model is developed to describe the heating and subsequent melting, vaporization and ionization of a target material during LIBS process. A numerical model based on one-dimensional thermal conductivity equation is being used to simulate the target evaporation and a hydrodynamic model is used to simulate plume expansion. Further, an experimental approach of measuring spectral emission from the ablation plume using emission spectroscopy and estimating the plasma state, such as the ionization species, and average plasma temperature, is investigated. An important result of this work is that for different ambient conditions, laser ablation plume dynamics can be estimated.     

Intense few-cycle laser pulses from self-compression in a self-guiding filament

Sub-10-fs-pulses are generated by self-compression in a noble gas filament. Using input pulses from a Ti:sapphire amplifier system with an energy of about 1.5 mJ at a repetition rate of 3 kHz and a pulse duration of 30 fs self-compressed sub-10-fs pulses with energies of about 0.3 mJ have been generated. These pulses are characterized with spectral phase interferometry for direct electrical-field reconstruction (SPIDER). Depending on the laser parameters, we observe a significant change in the chirp of the white-light. The spectral distribution of the outcoming beam profile is measured to distinguish the white-light core from the surrounding halo.     

224 nm segmented hollow-cathode silver ion laser

The segmented hollow-cathode discharge arrangement is used the first time to excite the 224 nm Ag II laser transition. Quasi-continuous output power of 45 mW is obtained during the 300 s current pulses at optimal discharge conditions (10 hPa of He+4% Ar buffer gas) for discharge current of 3 A. No power saturation is observed up to this current value. An average output power of 0.75 mW is reached using pulse repetition frequency of 190 Hz. The longitudinal mode structure of the TEM₀₀ transversal mode is measured by means of a scanning confocal Fabry–Perot interferometer. Two-mode operation is found to be dominant at high current values. Attempts and suggestions are made to prolong the lifetime of the laser tube. PACS 42.55.Lt; 42.60.Lh; 52.80.-s     

Tunable diode laser spectroscopy of benzene near 1684 nm with a low-temperature VCSEL

We describe the application of a long-wavelength vertical-cavity surface-emitting laser (VCSEL) with extended tuning range to the detection of benzene vapor at atmospheric pressure. A benzene absorption feature centered at 1684.24 nm was accessed by reducing the heat sink temperature of a VCSEL designed for room-temperature operation to −55°C. This allowed us to increase the injection current and thus to extend a single-scan tuning interval up to 46.4 cm⁻¹ or 13.2 nm around a central wavelength of 1687.4 nm. Five absorption lines of methane in the 5903–5950 cm⁻¹ range could be acquired within single laser scans at a repetition rate of 500 Hz. A benzene absorption feature between 5926 and 5948 cm⁻¹ was recorded for concentration measurements at atmospheric pressure using a single-pass 1.2 m absorption cell. A 50 ppmv mixture of CH₄ in N₂ was introduced into the cell along with benzene vapor to calibrate benzene concentration measurements. Benzene mixing ratios down to ∼90 ppmv were measured using a direct absorption technique. The minimum detectable absorbance and detection limit of benzene were estimated to be ∼10⁻⁴ and 30 ppmv, respectively. Using the wavelength modulation technique, we measured a second harmonic sensor response to benzene vapor absorption in air at atmospheric pressure as a function of modulation index. We conclude that a low-temperature monolithic VCSEL operating near 1684 nm can be employed in compact benzene sensors with a detection limit in the sub-ppm range.     

Sensitivity to anharmonicity of vibrational energy in a diatomic gasdynamic laser

A parameter for evaluating the sensitivity of quantum vibrational energy to anharmonicity in a diatomic gasdynamic laser is defined and calculated by considering the corresponding diatomic molecules as quantum anharmonic oscillators under an interatomic Morse potential. The variation of the above parameter in terms of the vibrational states and in terms of an involved anharmonic coefficient is discussed. In particular, the parameter in question at the classical limit is examined. Both weak and strong anharmonicities are discussed.     

High-repetition-rate high-beam-quality 43 W ultraviolet laser with extra-cavity third harmonic generation

High-power, high-repetition-rate extra-cavity third harmonic generation of 355 nm with high beam quality has been developed. The acoustic-optical Q-switched Nd:YVO₄ MOPA laser including 2- and 4-stage amplifiers was used as the IR source. With the extra-cavity frequency conversion of LBO crystals, 30.2 W TEM₀₀-mode 355 nm UV laser was obtained with a 2-stage amplifier MOPA laser, and the optical-to-optical (1064 nm to 355 nm) conversion efficiency was up to 30%. Enhanced 43 W TEM₀₀ UV laser at 60 kHz was achieved with a 4-stage amplifier MOPA IR laser, and pulse duration was 10.7 ns corresponding to the peak power as high as 67 kW, with single pulse energy of 0.72 mJ. The optical–optical efficiencies from IR and diodes to UV were 28% and 10% respectively.     

Femtosecond laser bonding of glasses and ion migration in the interface

We report femtosecond laser bonding with strengths of a few MPa and the material mixing during the laser bonding process by using Sm³⁺- and Cr³⁺-doped glasses and 180 fs pulses at a repetition rate of 1 kHz from an amplified Ti:sapphire laser at a wavelength of 785 nm. By analyzing fluorescence spectra taken around the interface using a confocal scanning microscope we observed the migration of Sm ions from the upper Sm-doped glass to the lower Cr-doped glass and the reduction from Sm³⁺ to Sm²⁺ ions just above the interface for the borate-borate material system. However, in Sm-doped borate-borosilicate, the laser bonding did not produce any reduction and migration of Sm³⁺ ions.     

A mid-infrared scanned-wavelength laser absorption sensor for carbon monoxide and temperature measurements from 900 to 4000 K

Mid-infrared laser absorption sensors based on quantum cascade laser (QCL) technology offer the potential for high-sensitivity, selective, and high-speed measurements of temperature and concentration for species of interest in high-temperature environments, such as those found in combustion devices. A new mid-infrared QCL absorption sensor for carbon monoxide and temperature measurements has been developed near the intensity peak of the CO fundamental band at 4.6 μm, providing orders-of-magnitude greater sensitivity than the overtone bands accessible with telecommunications lasers. The sensor is capable of probing the R(9), R(10), R(17), and R(18) transitions of the CO fundamental ro-vibrational band which are located at frequencies where H₂O and CO₂ spectral interference is minimal. Temperature measurements are made via scanned-wavelength two-line ratio techniques using either the R(9) and R(17) or the R(10) and R(18) line pairs. The high-speed (1–2 kHz) scanned-wavelength sensor is demonstrated in room-temperature gas cell measurements of CO and, to demonstrate the potential of the sensor for high-temperature thermometry, in shock-heated gases containing CO for a very wide range of temperature (950–3500 K) near 1 atm. To our knowledge, these measurements represent the first use of QCL-based absorption sensor for thermometry at elevated combustion-like temperatures. The high-temperature measurements of CO mole fraction and temperature agree with the post-reflected-shock conditions within ±1.5% and ±1.2% (1σ deviation), respectively.     

Evaluation of hybrid ytterbium–neodymium laser amplification at 1053 nm

We present here the modeling of a hybrid neodymium/ytterbium laser chain. The laser chain is modeled in energy, spectrum and gain for a relevant choice of ytterbium host materials. Special attention is given to spectral matching of both technologies. The model performance is benchmarked by an experimental setup of a Yb:glass regenerative-amplifier. Results indicate Yb:CaF₂ to be the best material for Nd:glass coupling.