厚原子蒸气介质中原子选择性光电离的理论研究

激光在厚原子蒸气介质中传播时会产生脉冲形变和延迟现象,这会直接影响原子多步光电离过程中的电离率和选择性.从原子蒸气激光同位素分离的实际出发,对厚原子蒸气介质中的原子光电离过程进行了研究,利用密度矩阵方法描述原子的光电离过程,利用Maxwell方程描述激光在厚介质中的传播,建立了介质中同时存在两种同位素的激光传播电离方程组,考察了原子蒸气参数和激光参数对厚介质中平均电离率和平均选择性的影响.研究结果表明:对于较厚的原子蒸气介质,激光功率的增加使平均电离率升高,平均选择性下降;对于相对较薄的介质,适当地降低激光功率可以同时提高平均电离率和平均选择性.存在一个正的激光延时使原子蒸气中目标同位素的平均电离率达到最大.尽量延长激光脉冲的宽度不仅可以同时提高目标同位素的平均电离率和平均选择性,还可以降低对激光脉冲之间相对延时的控制精度.     

Quantum state swap for two trapped Rydberg atoms

The quantum swap gate is one of the most useful gates for quantum computation. Two-qubit entanglement and a controlled-NOT quantum gate in a neutral Rydberg atom system have been achieved in recent experiments. It is therefore very interesting to propose a scheme here for swapping a quantum state between two trapped neutral atoms via the Rydberg blockade mechanism. The atoms interact with a sequence of laser pulses without individual addressing. The errors of the swap gate due to imprecision of pulse length, finite Rydberg interaction, and atomic spontaneous emission are discussed.     

量子统计权重对原子场电离效率的影响

原子能级的量子统计权重(G)是原子的重要光谱参数,但在研究原子的电离过程中通常却为了简化问题而被忽略.本文在锂原子的三步光激发(PE)+电场电离(EFI)过程中计入了其影响,并发现其对原子EFI效率的影响显著.本文精心设计了一套锂原子的PE+EFI方案:首先,采用三台不同波长的脉冲激光器分三步将原子从基态激发到某一Rydberg态上,经过一段时间延迟后再施加脉冲电场将其电离.针对原子所经历的PE、零场和EFI这三个物理过程,本文对其物理机制进行了分析并建立了服从粒子数守恒的物理模型进而导出了显含G参数的普适的速率方程组.其次,通过Matlab编程,分别针对精心选定的两条激发路径2S_(1/2)→2P_(1/2)→3S_(1/2)→25P_(1/2,3/2)和2S_(1/2)→2P_(3/2)→3D_(5/2)→25F_(5/2,7/2)开展了数值计算.研究发现:PE+EFI过程的总体效率的上限既与激光参数无关,也不依赖于G参数的绝对值,而是决定于Rydberg态的G参数的分支比.总之,通过精选激发路径可以调控PE过程各相关态的布居率,并能适当提高PE+EFI过程的总电离效率,但却因受到Rydberg态布居率的限制而很难进一步提高.     

Gain-switched semiconductor laser amplifier as an ultrafast dynamical optical gate

A gain-switched semiconductor laser is shown to act as an optical gate with picosecond resolution and amplification for light pulses from another laser source. The amplification mechanism and the gate width change qualitatively when the gate laser undergoes a transition from a pumping rate slightly below the dynamic laser threshold to slightly above the dynamic threshold. If the gate laser is pumped below but close to its dynamical threshold, unsaturated amplification of an external signal pulse occurs over a delay time range between the external optical pulse and the electrical driving pulse of about 100–200 ps which is equivalent to the optical gate width. The signal amplification is observed to increase by two orders of magnitude and the gate width decreases by one order of magnitude if the gate laser is pumped slightly above the dynamical threshold. Amplification then occurs for input signals injected much earlier. A detailed theory of coherent, time-dependent amplification including the nonlinear dynamics of the semiconductor laser is shown to account for the observations. Both amplification regimes, below and above threshold, are reproduced in the numerical simulations. The extremely short and highly sensitive gate range above threshold is identified as being due to the gain maximum related with the first relaxation oscillation of the laser.     

不同激光等离子体条件下的阿秒光脉冲产生

通过一维粒子模拟研究了利用相对论少周期强激光与固体密度等离子体表面相互作用实现单个孤立阿秒光脉冲产生的参数条件。主要研究描述相互作用的多维参数,如激光强度、入射角和等离子体标尺长度等,对相对论高次谐波能量转换效率和孤立阿秒光脉冲分离度的影响。研究发现,虽然激光等离子体参数对阿秒光脉冲产生的影响是复杂的,但是存在着能够实现大能量孤立阿秒光脉冲的最佳等离子体标尺长度和最佳入射角。当其他相互作用条件确定时,使用中等强度的相对论强激光可以在较宽的参数范围内实现孤立的阿秒光脉冲。大角度入射时,孤立阿秒光脉冲的分离度较高,能够实现孤立阿秒光脉冲的相互作用参数范围也较宽。     

A Noise-Robust Pulse for Excitation Transfer in a Multi-Mode Quantum Memory

Multi-mode quantum memory is a basic element required for long-distance quantum communication,as well as scalable quantum computation.For on-demand readout and long storage times,control pulses are crucial in order to transfer atomic excitations back and forth into spin excitations.Here,we introduce noise-robust composite pulse sequences for high-fidelity excitation transfer in multi-mode quantum memory.These pulses are robust to the deviations in amplitude and the detuning parameters of realistic conditions.We show the efficiency of these composite pulses with a typical rare-earth ion-doped system.This approach could be applied to a variety of quantum memory schemes.     

两束脉冲激光在级联的三能级系统中的传播

利用密度矩阵方程和麦克斯韦传播方程的耦合考虑激光脉冲的横向效应,在柱对称的条件下,研究了两束脉冲在级联系统中的共振传播,考察了脉冲在光学厚介质中的时空演化过程。数值计算中考虑了两个能级的自发辐射速度,给出了脉能量的空间演化及电熟粒子在空间的分布。     

Enhancing capacity of coherent optical information storage and transfer in a Bose-Einstein condensate

The coherent optical information storage capacity of an atomic Bose-Einstein condensate is examined. The theory of slow light propagation in atomic clouds is generalized to the short-pulse regime by taking into account group velocity dispersion. It is shown that the number of stored pulses in the condensate can be optimized for a particular coupling laser power, temperature, and interatomic interaction strength. Analytical results are derived for a semi-ideal model of the condensate using the effective uniform density zone approximation. Detailed numerical simulations are also performed. It is found that the axial density profile of the condensate protects the pulse against group velocity dispersion. Furthermore, taking into account the finite radial size of the condensate, multimode light propagation in an atomic Bose-Einstein condensate is investigated. The number of modes that can be supported by a condensate is found. The single-mode condition is determined as a function of experimentally accessible parameters including trap size, temperature, condensate number density, and scattering length. Quantum coherent atom-light interaction schemes are proposed for enhancing multimode light propagation effects.     

Pulsed laser ablation of GaAs using nano pulse length

Ablation using very short pulses has shown a great promise in facilitating the growth of complex multi-element films with stoichiometries matching those of their parent materials. GaAs is an important material in the electronic and opto-electronic industries and due to its compound structure it is an intriguing candidate for pulsed laser deposition. This work investigates the effect of nanosecond laser pulse lengths on the ablation of GaAs in an inert atmosphere. The number of pulses was varied in order to find the optimal condition for nano particles formation in our setup. The deposited structures were studied by grazing incidence small angle X-ray scattering and atomic force microscopy. It is shown that the GaAs nanoparticle sizes and size distributions can be controlled partly by the number of laser pulses applied in their production.     

短脉冲激光对硅基探测器的热作用模型选择

从傅里叶模型和非傅里叶模型的基本方程出发,通过有限差分方法对方程进行数值求解。分别分析了10,1．0,0．1,0．01 ns这4种脉宽的脉冲激光作用于硅材料时两种传热模型温度曲线的相对变化;讨论了热弛豫时间对非傅里叶模型数值结果的影响。结果表明:脉宽小于或等于100 ps的激光作用于硅材料时,表层温度上升缓慢,会发生载流子效应,非傅里叶模型可以合理地反映这种现象;对于一般材料,载流子效应发生的条件是脉宽小于或等于材料热弛豫时间,此时应当用非傅里叶模型描述加热过程。     

Effect of Pulse Width and Fluence of Femtosecond Laser on Electron--Phonon Relaxation Time

The electron phonon relaxation time as functions of pulse width and fluence of femtosecond laser is studied based on the two-temperature model. The two-temperature model is solved using a finite difference method for copper target. The temperature distribution of the electron and the lattice along with space and time for a certain laser fluence is presented. The time-dependence of lattice and electron temperature of the surface for different pulse width and different laser fluence are also performed, respectively. Moreover, the variation of heat-affected zone per pulse with laser Auence is obtained. The satisfactory agreement between our numerical results and experimental data indicates that the electron-phonon relaxation time is reasonably accurate with the influences of pulse width and Auence of femtosecond laser.     

Propagation of elliptically polarized laser pulses in isotropic gyrotropic medium with relaxation cubic nonlinearity and anomalous frequency dispersion

The self-action of elliptically polarized Gaussian laser pulses in an isotropic gyrotropic medium with an anomalous frequency dispersion and cubic Kerr nonlinearity with a finite relaxation time on the order of the pulse duration is numerically studied. It is shown that, at the output of the medium, the pulse polarization nonmonotonically varies with time. The main peak of the pulse is additionally delayed compared to the time of passing the linear medium; the value of this delay significantly depends on the polarization of the incident pulse and achieves a maximum for incident pulses whose degree of ellipticity is equal to the ratio of the material constants characterizing the local and nonlocal nonlinear optical response of the medium. It seems promising to search for possible differences in relaxation times depending on the intensity of additions to the refractive indices of the right and left circularly polarized waves by investigating the time dependence of polarization characteristics at the output of the medium.     

Parametric study of plasma active medium and gain saturation region in a Ne-like soft X-ray laser

Plasmas created by the interaction of high power optical laser with a target surface can be used as a source of soft X-ray lasers. Plasma and pump laser characteristics play significant role in achieving high gain coefficient for such plasma based on soft X-ray lasers. In the present work, the plasma active medium parameters for germanium element at a wavelength of 19.6 nm irradiated by a double-pulse pump laser have been studied using MED103 hydrodynamic code. For this purpose, first, the effects of laser intensity, pulse width and delay time of two pulses on the gain coefficient have been investigated and the optimum conditions for the maximum gain extent of Ne-like germanium soft X-ray laser are obtained. Then, in order to calculate the intensity of such high gain lasers in which Linford equation is invalid, we have adopted the general formula of amplified spontaneous emission intensity, which is valid in all range of intensities even at much higher intensities than saturation intensity. Finally, the soft X-ray laser intensities in the saturated areas for different plasma lengths have been calculated. The results show that the output of soft X-ray laser intensity with 294 cm⁻¹ gain coefficient can reach to about several times saturated intensity by applying a 1–2 mm plasma length as the active medium.     

波长可调谐超短光脉冲的简便高质的生成技术

提出了一种以处于增益开关调制状态下的法布里珀罗(Fabry-Pérot)半导体激光器作为光源,采用简单的自激注入锁定方式,以生成波长可调谐的超短光脉冲的实验系统。该实验装置中,激光器的外腔包括两个串联在一起的布拉格光纤光栅,一个掺铒光纤放大器(EDFA),一个光耦合器和两个环行器,其作用是选模,以及增强并控制反馈回激光器内腔的光强。该实验系统简单而高效,在24nm的波长调谐范围内获得了边模抑制比高于40dB的单模光脉冲输出;而在1521.8nm和1550.0nm之间28.2nm的波长调谐范围内,边模抑制比高于35dB。所得到的各个单波长激光脉冲的时域半峰全宽为140~260ps,各个脉冲的光谱半峰全宽皆为0.1nm。     

Theory of the statistical properties of ultra-short pulses generated by a passively mode-locked solid-state laser

The evolution of ultra-short pulses from noise in a passively mode-locked solid-state laser is treated. The statistical properties of the laser field, such as correlation functions, the mean pulse shape and its fluctuations, are investigated. The maximum intensity and the width of the pulse train are estimated taking account of the amplification saturation. As an example of the application of the results to non-linear optics, TPF traces are calculated.     

Suppression of gain narrowing in multi-TW lasers with negatively and positively chirped pulse amplification

A laser scheme implementing a combination of negatively and positively chirped pulse amplification (NPCPA) is demonstrated. This method of amplification suppresses spectral narrowing typically appearing in chirped pulse amplification (CPA) lasers thus supporting pulse spectrum much broader than a conventional CPA. With a NPCPA Ti:Sapphire laser we have achieved laser pulses of 50 nm spectral width and 150 mJ energy without any additional spectral correction. The scheme appears as an easy and reliable solution to preserve spectral bandwidth in Ti:Sapphire lasers, especially at high power levels up to the Petawatt regime. PACS 42.60 By, Lh; 42.65 Re     

Experimental study of an all-fiber laser actively mode-locked by standing-wave acousto-optic modulation

We report an experimental study of an actively mode-locked erbium-doped all-fiber laser, based on a standing-wave acoustically-induced superlattice modulation. Our experiments involve the characterization of the laser as a function of the active fiber length, and with different types of delay line fibers. The effect of the modulation on the laser performance was also investigated. Narrower pulses were obtained at higher modulation depths, normal dispersion, and shorter lengths of active fiber. Optical pulses of 160 mW peak power and 630 ps temporal width were obtained at 9 MHz repetition rate.     

Analytical model for ion acceleration by high-intensity laser pulses

We present a general expression for the maximum ion energy observed in experiments with thin foils irradiated by high-intensity laser pulses. The analytical model is based on a radially confined surface charge set up by laser accelerated electrons on the target rear side. The only input parameters are the properties of the laser pulse and the target thickness. The predicted maximum ion energy and the optimal laser pulse duration are supported by dedicated experiments for a broad range of different ions.     

1064nm纳秒激光脉冲激发的外腔式PbWO4拉曼激光器

研究了外腔式PbWO4拉曼激光器在纳秒脉冲抽运下的输出特性。利用主动调Q的Nd:YAG激光器产生的脉冲宽度为31.4ns,最大输出能量为200mJ的1064nm激光作为抽运源。拉曼激光谐振腔采用的是平凹腔设计。测量了输出的拉曼光脉宽与抽运能量的关系,分析了输出的拉曼光脉冲波形图和光谱图,测量了输出的拉曼光脉冲能量与抽运能量的关系,计算了转换效率与抽运能量的关系。当注入抽运光能量达到42mJ时,得到了一阶斯托克斯光脉冲的最大能量和转换效率分别为10mJ和24%,获得外腔式PbWO4拉曼激光器的一阶斯托克斯光脉冲波长为1177.6nm,典型的一阶斯托克斯光脉冲脉宽为20ns。     

Optical rectification of highly focused near-IR pulses in the plasmon waveguide

Generation of terahertz pulses via mixing the Fourier harmonics of strongly focused near-IR pumping laser pulses in a plasmon waveguide filled with a nonlinear medium is considered. At a certain choice of its parameters, this waveguide provides efficient transverse confinement of the terahertz mode and a low dispersion of its refractive index. As a result, the system becomes capable of generating short fairly intense terahertz pulses. Such an approach significantly (by a factor of 50) decreases the pump power compared with that in the conventional (waveguide-free) schemes, which generate terahertz pulses from single pumping pulses (optical rectification), and still yields the same intensity of the output terahertz pulse and conversion efficiency. For the Ag-GaP-Ag structure taken as an example, optimal parameters of the plasmon waveguide and pumping pulse are found and characteristics of the output terahertz pulse are calculated.