Level structure of 99Rh at high spins

High spins states in ⁹⁹Rh were populated via the ⁶⁶Zn(³⁷Cl, 2p2n)⁹⁹Rh reaction at an incident beam energy of 130 MeV. Seventeen new transitions have been observed in the present study and the level scheme has now been extended up to a spin of J∼ 25ħ and an excitation energy of about E _x∼ 10 MeV. The observation of a positive parity E2 cascade based on the 9/2⁺ isomeric level is suggestive of collective behaviour in this nucleus up to high spins. Spherical shell model (within restricted model space) and Cranked shell model calculations were performed to obtain an insight into the observed level structure. The new collective band observed up to a spin of J∼ 25ħ is suggested to be based on (πg _9/2 ³) ⊗ (νg _7/2 ²) quasi-particle excitations. Received: 12 July 1999 / Revised version: 14 September 1999     

Structure of 136Te and the problem of mass of 134Te

Neutron-rich, N=84 nuclei from the ₁₃₂Sn region, populated in spontaneous fission of ₂₄₈Cm, have been studied with EUROGAM 2. Excited states and their spins and parities in the ₁₃₆Te nucleus were established up to 17ħ. OXBASH code calculations support the experimental identification of maximum aligned configurations in ₁₃₆Te. Empirical shell model calculations for the I_π= 14₊ level in ₁₃₆Te indicate that the adopted mass of the ₁₃₄Te nucleus should be lowered by 200(80) keV. Received: 3 August 1998     

Lifetimes and configuration mixing in 110Cd

Lifetimes of excited states in ¹¹⁰Cd have been measured by the Doppler shift attenuation method in the reaction (α,2nγ) at E _α= 25 MeV. Lifetime values for 8 states and lifetime limits for 3 states were obtained. The band structures of ¹¹⁰Cd have been interpreted in terms of a modified version of the interacting boson model (IBM + 2 q.p.). The calculations explain well the excitation energies and electromagnetic transition probabilities up to J ^π= 16⁺, except for the 10⁺ ₁ state. The structural features are discussed in terms of collective and two quasiparticle excitations. Received: 20 March 1999 / Revised version: 28 May 1999     

High-spin structure of the neutron-rich 107,109 45Rh isotopes: the role of triaxiality

The ^107,109Rh nuclei have been produced as fission fragments following the fusion reaction ²⁸Si +¹⁷⁶Yb at 145 MeV bombarding energy and studied with the Eurogam2 array. In both nuclei three new rotational bands with the odd proton occupying the πg_9/2, πp_1/2 and π(g_7/2/d_5/2) sub-shells have been observed. In ¹⁰⁷Rh, two other bands involving strong M1 transitions have been identified at excitation energy larger than 2 MeV. They can be interpreted in terms of three quasiparticle excitations. In addition new structures consisting of four transitions, built on states located at low excitation energy (680 keV in ¹⁰⁷Rh and 642 keV in ¹⁰⁹Rh), point out the importance of triaxial deformation in these two isotopes. Received: 1 September 1999     

New nuclide 139Tb and (EC +β+) decay of 138,139Gd

Excited levels in ¹³³Sn and ¹³⁴Sb, populated in spontaneous fission of ²⁴⁸Cm, were studied by means of prompt-γ spectroscopy, using the EUROGAM 2 multidetector array. The neutron i _13/2 single-particle energy has been determined for the first time in the ¹³²Sn region. The energy of the h _9/2 neutron level, proposed previously, has been confirmed. Received: 13 January 1999 / Revised version: 22 March 1999     

A new high-spin isomer in 145Sm

A new high-spin isomer in ¹⁴⁵Sm was observed by in-beam γ-ray spectroscopy with the reaction ¹²²Sn(²⁷Al,3np) at 127 MeV performed at the Nordball multi-detector array in Roskilde. The excitation energy of the isomer was determined to be E _x= 11147 keV, and using the generalized centroid-shift method its half-life was found to be T _1/2= (7.4 ± 1.0) ns. Received: 23 October 1998     

High-spin structures observed in the 101Tc fission fragment

High-spin states have been studied in ¹⁰¹Tc produced as a fission fragment in the reaction ¹⁷⁶Yb +²⁸Si at 145 MeV. Gamma rays were detected with the EUROGAM2 array. The level scheme of ¹⁰¹Tc has been extended up to 4.2 MeV excitation energy and several band structures are observed. Configurations are assigned to two new bands on the basis of their behaviour and of cranked Hartree-Fock-Bogolyubov calculations. Received: 4 January 1999     

The low-spin structure of <Superscript>115</Superscript>Xe

The low-spin band structure of neutron-deficient ¹¹⁵ ₅₄Xe has been studied following a low-energy (212.3 MeV) ⁶⁰Ni(⁵⁸Ni,2pnγ) reaction performed at IReS, Strasbourg, with the Garel⁺ spectrometer. The relative excitation energies of νh_11/2 (isomeric), νg_7/2, and νd_5/2 bandheads have been established. Received: 23 March 2000     

Yrare bands of 121Xe

High-spin states in ¹²¹Xe have been studied via the ¹⁰⁹Ag (16O, p3n) ¹²¹Xe reaction at a beam energy of 80 MeV. Several rotational bands based on one- and three-quasiparticle excitations have been established. Among them, an unfavoured yrare rotational band with unfavoured signature has been newly identified. Received: 19 November 1998     

Systematics of related high-spin isomers in 144Sm and other N = 82 nuclei

An in-beam experiment with the reaction ¹²²Sn(²⁷Al,4np) at 127 MeV was performed at the Nordball multi-detector array in Roskilde. It provided evidence for a new high-spin isomer in ¹⁴⁴Sm. This isomer with T _1/2= (2.6 ± 0.5) ns at an excitation energy E _x= 9232 keV seems to belong to a family of isomers of similar configuration in neighbouring N= 82 nuclei. Received: 16 November 1997     

Super-allowed α decay above doubly-magic <Superscript>100</Superscript>Sn and properties of <Superscript>104</Superscript>Te = <Superscript>100</Superscript>Sn ⊗ α

α-decay half-lives for ^{104, 105, 106}Te and ^{108, 109, 110}Xe close above the doubly-magic ¹⁰⁰Sn are calculated from systematic double-folding potentials. The derived α preformation factors are compared to results for ^{212, 213, 214}Po and ^{216, 217, 218}Rn above the doubly-magic ²⁰⁸Pb. α-decay energies of Q _α = 5.42±0.07MeV and 4.65±0.15MeV are predicted for ¹⁰⁴Te and ¹⁰⁸Xe; the corresponding half-lives are T _1/2 ≈ 5ns for ¹⁰⁴Te and of the order of 60μs for ¹⁰⁸Xe. Additionally, the properties of rotational bands in ¹⁰⁴Te are analyzed, and the first excited 2⁺ state in ¹⁰⁴Te is predicted at E _x = 650±40keV; it decays preferentially by γ emission with a reduced transition strength of 10 Weisskopf units to the ground state of ¹⁰⁴Te and with a minor branch by α emission to the ground state of ¹⁰⁰Sn.     

γ Spectroscopy of 209Pb with deep inelastic reactions

High spin states in nuclei around ²⁰⁸Pb were populated in deep inelastic collisions of ⁷⁶Ge, ¹³⁶Xe, and ²⁰⁸Pb projectiles with ²⁰⁸Pb targets at beam energies about 12% above the Coulomb barrier. New states in ²⁰⁹Pb were found by measuring γ-γ-coincidences. They are interpreted as the yrast states that originate from the coupling of one neutron to the lowest excitations of the ²⁰⁸Pb core. The results are discussed in the frame of the shell model. Received: 22 November 1997     

Physics with heavy neutron-rich RIBs at the HRIBF

The Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory has recently produced the world's first post-accelerated beams of heavy neutron-rich nuclei. The first experiments with these beam are described, and the results discussed. B(E2;0⁺ → 2⁺) values for neutron-rich ^126,128Sn and ^132,134,136Te isotopes have been measured by Coulomb excitation in inverse kinematics. The results for ¹³²Te and ¹³⁴Te (N = 80, 82) show excellent agreement with systematics of lighter Te isotopes, but the B(E2) value for ¹³⁶Te (N = 84) is unexpectedly small. Single-neutron transfer reactions with a ¹³⁴Te beam on ^natBe and ¹³C targets at energies just above the Coulomb barrier have also been studied. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: radford@mail.phy.ornl.gov     

Configuration assignments and decay of 126La high-spin bands

High spin states of ¹²⁶La have been populated using the reaction ¹¹⁶Sn+¹⁴N at 68 MeV. γ-rays and conversion electrons were detected with the GAREL array. Multipolarities of the lowest-lying in-band dipole transitions have been determined from the deduced internal conversion coefficients. Experimental B(M1)/B(E2) ratios have been derived for the bands and compared with calculated values using the D?nau-Frauendorf geometrical model. Configurations are proposed for the bands comparing them with cranked shell model calculations and on the basis of the measured B(M1)/B(E2) ratios. The β-decay of ¹²⁶La has also been revisited. The population of the ¹²⁶Ba levels gives a probable spin value of five for the decaying high-spin ¹²⁶La state with T _1/2≈ 64 s which may indicate a signature inversion in the πh_11/2νh_11/2 band. Received: 12 October 1999     

High spin states and evidence for octupole correlations in 117Xe

High-spin states of ¹¹⁷Xe were investigated by means of in-beam γ-ray spectroscopic techniques via the reaction of ²⁸Si bombarding a ⁹²Mo target at beam energies of 100-120 MeV. A positive-parity rotational band decaying into the yrast negative-parity band by a series of enhanced E1 transitions was observed for the first time, implying the existence of octupole correlations in ¹¹⁷Xe. The B(E1) values increase with spin. The νd_5/2 band was firmly established up to 27/2⁺ and the B(M1)/B(E2) ratios were extracted from the relative intensities of γ-rays in this band. The previously known νh_11/2 and νg_7/2 [413]5/2⁺α=−1/2 bands were confirmed and extended up to high spins and two bandcrossings are observed in the latter at ħω=0.33 and 0.44 MeV, respectively. The bandcrossings and configurations of these bands are discussed by TRS and CSM calculations. In a γ–γ–t measurement, the 11/2⁻ and 7/2⁻ levels were identified as two isomers with half-lives of 59.4±20 ns and 16.5±8.0 ns, respectively. Received: 17 June 1997 / Revised version: 29 September 1997     

New states in heavy Cd isotopes and evidence for weakening of the N = 82 shell structure

A chemically selective laser ion source has been used in a β-decay study of heavy Ag isotopes into even-even Cd nuclides. Gamma-spectroscopic techniques in time-resolving event-by-event and multiscaling modes have permitted the identification of the first 2⁺ and 4⁺ levels in ¹²⁶Cd₇₈, ¹²⁸Cd₈₀, and tentatively the 2⁺ state in ¹³⁰Cd₈₂. From a comparison of these new states in ₄₈Cd with the E(2⁺) and E(4⁺)/E(2⁺) level systematics of ₄₆Pd and ₅₂Te isotopes and several recent model predictions, possible evidence for a weakening of the spherical N = 82 neutron-shell below double-magic ¹³²Sn is obtained. Received: 13 July 2000 / Accepted: 12 October 2000     

First observation of excited states in 197At: the onset of deformation in neutron-deficient astatine nuclei

Excited states in the Z= 85 nucleus ¹⁹⁷At have been identified for the first time using the recoil-decay-tagging (RDT) technique. The excitation energy of these states is found to be consistent with the systematics of neutron-deficient astatine nuclei and with theoretical calculations indicating that the nucleus may be deformed in its ground state. Received: 8 January 1999     

Simplex s = ±i excitations in 141Xe

Excited levels in ¹⁴¹Xe, populated in spontaneous fission of ²⁴⁸Cm, were studied by means of prompt -ray spectroscopy, using the EUROGAMM2 array. Level scheme of ¹⁴¹Xe obtained in this work shows patterns characteristic of simplex symmetry with s=+i and s=-i bands present but low value of D₀ moment indicates that octupole correlations in Xe isotopes are systematically lower than in Ba nuclei. Received: 9 March 2000 / Accepted: 4 May 2000     

GCM analysis of the collective properties of lead isotopes with exact projection on particle numbers

We present a microscopic analysis of the collective behaviour of the lead isotopes in the vicinity of ²⁰⁸Pb. In this study, we rely on a coherent approach based on the Generator Coordinate Method (GCM) including exact projection on N and Z numbers within a collective space generated by means of the constrained Hartree-Fock BCS method. With the same Hamiltonian used in HF + BCS calculations, we have performed a comprehensive study including monopole, quadrupole and octupole excitations as well as pairing vibrations. We find that, for the considered nuclei, the collective modes which modify the most the conclusions drawn from the mean-field theory are the octupole and pairing vibrations. Received: 31 May 2001 / Accepted: 23 August 2001