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Field-Free Molecular Orientation Generated from Cyclic Rotational States by Using Two Trains of Half-Cycle Pulses
作者姓名:黄宇欣  杨玉军  朱红玉  王丽  王晖  朱颀人
作者单位:[1]Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012 [2]Institute of Theoretical Chemistry, Jilin University, Changchun 130012
基金项目:Supported by the National Natural Science Foundation of China under Grant No 10474028, the Specialized Research Fund for the Doctoral Programme of Higher Education of China under Grant No 20040183041, and the Research Fund for the Innovative Project of Jilin University.
摘    要:We show that two trains of half-cycle pulses (HCPs) with different amplitudes irradiating alternately on polar molecules can achieve a remarkable enhancement of field-free orientation compared with the case of an equal amplitude HCPs train for the same pulse separation. optimal adjustment of the population distribution on This kind of orientation enhancements is mainly due to an every field-free angular momentum eigenstate, in which the populations on the undesired states of high angular momenta are effectively suppressed, and the populations on the desired states of low angular momenta are correspondingly promoted.

关 键 词:分子状态  循环旋转  原子核  相互作用
收稿时间:2007-04-02

Field-Free Molecular Orientation Generated from Cyclic Rotational States by Using Two Trains of Half-Cycle Pulses
HUANG Yu-Xin,YANG Yu-Jun,ZHU Hong-Yu,WANG Li,WANG Hui,ZHU Qi-Ren.Field-Free Molecular Orientation Generated from Cyclic Rotational States by Using Two Trains of Half-Cycle Pulses[J].Chinese Physics Letters,2007,24(11):3111-3114.
Authors:HUANG Yu-Xin  YANG Yu-Jun  ZHU Hong-Yu  WANG Li  WANG Hui  ZHU Qi-Ren
Affiliation:Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012 Institute of Theoretical Chemistry, Jilin University, Changchun 130012
Abstract:We show that two trains of half-cycle pulses (HCPs) with different amplitudes irradiating alternately on polar molecules can achieve a remarkable enhancement of field-free orientation compared with the case of an equal amplitude HCPs train for the same pulse separation. This kind of orientation enhancements is mainly due to an optimal adjustment of the population distribution on every field-free angular momentum eigenstate, in which the populations on the undesired states of high angular momenta are effectively suppressed, and the populations on the desired states of low angular momenta are correspondingly promoted.
Keywords:32  80  Lg  02  30  Yy  33  80  -b
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