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Polarized photoluminescence spectroscopy in WS2, WSe2 atomic layers and heterostructures by cylindrical vector beams
Affiliation:1.Key Laboratory for Micro-Nano Physics and Technology of Hunan Province, School of Physics and Electronics, Hunan University, Changsha, Hunan 410082, China;2.Institute of Physical and Theoretical Chemistry and LISA+, University of Tübingen, Auf der Morgenstelle 18, 72076, Tübingen, Germany;3.College of Materials Science and Engineering, Hunan University, Changsha, Hunan 410082, China
Abstract:Due to the large exciton binding energy, two-dimensional (2D) transition metal dichalcogenides (TMDCs) provide an ideal platform for studying excitonic states and related photonics and optoelectronics. Polarization states lead to distinct light-matter interactions which are of great importance for device applications. In this work, we study polarized photoluminescence spectra from intralayer exciton and indirect exciton in WS2 and WSe2 atomic layers, and interlayer exciton in WS2/WSe2 heterostructures by radially and azimuthally polarized cylindrical vector laser beams. We demonstrated the same in-plane and out-of-plane polarization behavior from the intralayer and indirect exciton. Moreover, with these two laser modes, we obtained interlayer exciton in WS2/WSe2 heterostructures with stronger out-of-plane polarization, due to the formation of vertical electric dipole moment.
Keywords:two-dimensional transition metal dichalcogenides  optical polarization  interlayer exciton  cylindrical vector beams  
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