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Precise measurement of the line width of the photoassociation spectra of ultracold molecules by using a frequency shifter
Authors:Wu Ji-Zhou   Ma Jie    Ji Zhong-Hua    Zhang Yi-Chi   Li Yu-Qing    Wang Li-Rong    Zhao Yan-Ting   Xiao Lian-Tuan    Jia Suo-Tang
Affiliation:State Key Laboratory of Quantum Optics and Quantum Optics Devices, Laser Spectroscopy Laboratory, College of Physics and Electronic Engineering, Shanxi University, Taiyuan 030006, China
Abstract:We propose a technique to precisely measure the line width of the photoassociation spectra of the excited cesium molecule by using a frequency shifter to generate two laser beams with a precise frequency difference. A series of photoassociation (PA) spectra are recorded with two laser beam induced molecular lines, whose peak separation serves as an accurate frequency ruler to measure the line width of the PA spectra. The full width half maximum line width was studied as a function of PA laser intensity. The extrapolated value at zero laser intensity is (34.84 ± 0.22) MHz. By analyzing other broadening mechanisms, a value of (32.02 ± 0.70) MHz was deduced. It is shown that this scheme is inexpensive, simple, robust, and is promising for applications in a variety of other atomic species.
Keywords:laser cooling   molecular spectroscopy   line shapes and width
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