Wood‐Derived Ultrathin Carbon Nanofiber Aerogels |
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Authors: | Si‐Cheng Li Bi‐Cheng Hu Dr Yan‐Wei Ding Prof Hai‐Wei Liang Chao Li Dr Zi‐You Yu Dr Zhen‐Yu Wu Prof Wen‐Shuai Chen Prof Shu‐Hong Yu |
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Affiliation: | 1. http://staff.ustc.edu.cn/~yulab/;2. Division of Nanomaterials & Chemistry, Hefei National Research Center for Physical Sciences at the Microscale, Collaborative Innovation Center of Suzhou Nano Science and Technology, Department of Chemistry, CAS Center for Excellence in Nanoscience, Hefei Science Center of CAS, University of Science and Technology of China, Hefei, Anhui, P. R. China;3. Key laboratory of Bio-based Material Science and Technology, Ministry of Education, Northeast Forestry University, Harbin, P. R. China |
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Abstract: | Carbon aerogels with 3D networks of interconnected nanometer‐sized particles exhibit fascinating physical properties and show great application potential. Efficient and sustainable methods are required to produce high‐performance carbon aerogels on a large scale to boost their practical applications. An economical and sustainable method is now developed for the synthesis of ultrathin carbon nanofiber (CNF) aerogels from the wood‐based nanofibrillated cellulose (NFC) aerogels via a catalytic pyrolysis process, which guarantees high carbon residual and well maintenance of the nanofibrous morphology during thermal decomposition of the NFC aerogels. The wood‐derived CNF aerogels exhibit excellent electrical conductivity, a large surface area, and potential as a binder‐free electrode material for supercapacitors. The results suggest great promise in developing new families of carbon aerogels based on the controlled pyrolysis of economical and sustainable nanostructured precursors. |
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Keywords: | carbon nanofiber aerogels nanofibrillated cellulose pyrolysis chemistry supercapacitors wood |
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