Abstract: | Sufficient conditions for the convergence in distribution of an infinite convolution product of measures on a connected Lie group with respect to left invariant Haar measure are derived. These conditions are used to construct distributions that satisfy where is a refinement operator constructed from a measure and a dilation automorphism . The existence of implies is nilpotent and simply connected and the exponential map is an analytic homeomorphism. Furthermore, there exists a unique minimal compact subset such that for any open set containing and for any distribution on with compact support, there exists an integer such that implies If is supported on an -invariant uniform subgroup then is related, by an intertwining operator, to a transition operator on Necessary and sufficient conditions for to converge to , and for the -translates of to be orthogonal or to form a Riesz basis, are characterized in terms of the spectrum of the restriction of to functions supported on |