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化学进展 2022, Vol. 34 Issue (4): 950-962 DOI: 10.7536/PC210442 前一篇   后一篇

• 综述 •

磁性NiFe2O4基复合材料的构筑及光催化应用

李晓微1, 张雷2,*(), 邢其鑫1, 昝金宇1, 周晋1, 禚淑萍1   

  1. 1 山东理工大学化学化工学院 淄博 255000
    2 安徽理工大学材料科学与工程学院 淮南 232001
  • 收稿日期:2021-04-22 修回日期:2021-07-27 出版日期:2022-04-24 发布日期:2021-07-29
  • 通讯作者: 张雷
  • 基金资助:
    国家自然科学基金项目(51502162); 国家自然科学基金项目(21975001); 安徽省高等学校自然科学研究项目(KJ2019A0115); 山东理工大学青年教师发展支持计划资助
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Construction of Magnetic NiFe2O4-Based Composite Materials and Their Applications in Photocatalysis

Xiaowei Li1, Lei Zhang2(), Qixin Xing1, Jinyu Zan1, Jin Zhou1, Shuping Zhuo1   

  1. 1 School of Chemistry and Chemical Engineering, Shandong University of Technology,Zibo 255000, China
    2 School of Materials Science and Engineering, Anhui University of Science and Technology,Huainan 232001, China
  • Received:2021-04-22 Revised:2021-07-27 Online:2022-04-24 Published:2021-07-29
  • Contact: Lei Zhang
  • Supported by:
    National Natural Science Foundation of China(51502162); National Natural Science Foundation of China(21975001); Key Project of Natural Science Research for Colleges and Universities of Anhui Province of China(KJ2019A0115); Young Teacher Supporting Fund of Shandong University of Technology

随着社会经济的快速发展,能源短缺与环境污染已成为当前人类面临的两大难题。人们一直致力于开发新的清洁可再生替代能源, 其中,太阳能被认为是理想且具有发展潜力的清洁能源。光催化作为一种新型的“绿色技术”,可直接利用太阳能将环境中的有机污染物降解为无害物质,进而有效解决上述问题。然而,要实现这个过程关键在于合理地设计和构筑高性能的光催化剂。铁酸镍(NiFe2O4)作为一种磁性材料,兼具快速的磁响应性和良好的光化学稳定性,将其与能带匹配的半导体光催化剂复合,不仅能够获得活性高的光催化剂,而且实现了光催化剂的磁分离, 从而使其在光催化领域展现出极为广阔的应用前景。本文主要综述了近5年来国内外NiFe2O4基复合材料的制备和光催化应用方面的最新研究进展, 这将为新型高效磁性复合光催化材料的合成及应用提供新方法和新思路。最后,对NiFe2O4基复合光催化材料未来的发展前景做了展望。

关键词： 铁酸镍, 磁性, 复合材料, 光催化

Environmental pollution and energy shortage caused by the rapid development of the economy have become two major problems in modern society. Accordingly, much research is currently focused on the exploitation of new alternative energy sources. Among various energy sources, solar energy is considered to be ideal and renewable energy. Under sunlight irradiation, photocatalysis, as a novel “green technology”, can directly convert organic pollutants into innoxious substances to solve both energy crisis and environmental pollution. However, the key to the success of this process is dependent on the rational design and fabrication of efficient photocatalysts. The NiFe2O4 possessing fast magnetism response and good photochemistry stability, is coupled with other semiconductor photocatalysts having a suited band gap in order to obtain greatly effective photocatalytic systems and achieve the magnetic separation, exhibiting wide application foreground. This paper mainly reviews the latest research progress on the synthesis and photocatalytic application of NiFe2O4-based composites, which may open a new avenue and idea for preparing highly active and magnetically separable composite photocatalysts. Finally, the future development of NiFe2O4-based photocatalytic materials is also prospected.

Contents

1 Introduction

2 NiFe2O4/carbon materials

2.1 NiFe2O4/graphene

2.2 NiFe2O4/g-C3N4

2.3 NiFe2O4/other carbon materials

3 NiFe2O4/Bismuth-based compounds

3.1 NiFe2O4/BiOX

3.2 NiFe2O4/Aurivillius Bismuth-based oxide

3.3 NiFe2O4/other Bismuth-based compounds

4 NiFe2O4/Silver-based compounds

4.1 NiFe2O4/Ag3PO4

4.2 NiFe2O4/AgX

5 NiFe2O4/TiO2

6 NiFe2O4/ZnO

7 Conclusion and outlook

Key words: NiFe2O4, magnetic, composites, photocatalysis
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图1 NiFe2O4-RGO光催化降解MB的机理示意图[24]
Fig. 1 Mechanism of photocatalytic degradation of MB in the presence of NiFe2O4-RGO[24]
图2 g-C3N4/NiFe2O4的直接Z型光催化机理[35]
Fig. 2 The proposed direct Z-scheme photocatalytic mechanism for the g-C3N4/NiFe2O4 nanocomposite[35]
图3 g-C3N4/graphene/NiFe2O4的全固态Z型光催化机理[39]
Fig. 3 The proposed all-solid-state Z-scheme photocatalytic mechanism for the g-C3N4/graphene/NiFe2O4 nanocomposite[39]
图4 (a,b) NiFe2O4/C的SEM图,(c) TEM图,(d) HRTEM图[40]
Fig. 4 (a,b) SEM images,(c) TEM image and (d) HRTEM image of NiFe2O4/C[40]
表1 不同NiFe2O4/碳材料复合光催化降解污染物的性能对比
Table 1 The photocatalytic activity of pollutant degradation over different NiFe2O4/carbon material composites
Photocatalyst Pollutant Degradation efficiency (%) Degradation
time(min)		 Light condition ref
NiFe2O4-RGO Methylene blue 20 mg/L ~99.1 180 800 W Xe lamp, visible light 24
NiFe2O4@GO Methylene blue 0.04 mmol/L ~100 120 10 W UV lamp, UV light 25
2%NiFe2O4/g-C3N4 Methyl orange 10 mg/L ~68 60 300 W Xe lamp, visible light 33
NiFe2O4-g-C3N4 Methylene blue 20 mg/L ~98 225 40 W LED bulb, visible light 34
NiFe2O4-g-C3N4 Rhodamine B 10 mg/L ~90 225 40 W LED bulb, visible light 34
NiFe2O4-g-C3N4 Methylene blue 20 mg/L ~99 225 direct sunlight 34
NiFe2O4-g-C3N4 Rhodamine B 10 mg/L ~99 225 direct sunlight 34
g-C3N4/NiFe2O4 Methyl orange 10 mg/L ~100 210 10 W LED lamp, visible light 35
g-C3N4/NiFe2O4-12% Methylene blue 50 mg/L ~100 75 300 W Xe lamp, visible light 36
Boron doped g-C3N4/NiFe2O4 Methylene blue 5 mg/L ~98 80 350 W Mercury-Xenon lamp 37
20%NiFe2O4@P-g-C3N4 Phenol 20 mg/L ~96 60 Direct sunlight 38
20%NiFe2O4@P-g-C3N4 Hydrogen production ~904 μmol/h 150 W Xe arc lamp, visible light 38
g-C3N4/graphene/NiFe2O4-25% Methyl orange 10 mg/L ~100 120 10 W LED lamp, visible light 39
NiFe2O4/C Tetracycline hydro chloride 20 mg/L ~97.25 60 800 W Xe lamp, visible light 40
25%NiFe2O4-MWCNT Sulfamethoxazole 5 mg/L ~100 120 100 W mercury lamp, UV-A light 41
图5 (a,b) NiFe2O4/BiOBr的TEM图[53]
Fig. 5 (a,b) TEM images of NiFe2O4/BiOBr[53]
图6 (a) NiFe2O4/BiOBr的TEM图; (b) NiFe2O4/BiOBr的HRTEM图[54]
Fig. 6 (a) TEM image of NiFe2O4/BiOBr; (b) HRTEM image of NiFe2O4/BiOBr[54]
图7 NiFe2O4/BiOI的能带结构和可能的电荷迁移路径[56]
Fig. 7 Band structure and possible photogenerated charges migration path of NiFe2O4/BiOI nanocomposite[56]
图8 Ag3PO4/Ag/NiFe2O4光催化降解MB的反应机理[81]
Fig. 8 Photocatalytic mechanism of MB degradation by Ag3PO4/Ag/NiFe2O4 composite[81]
图9 (a,b) Ag3PO4/GO/NiFe2O4的SEM图[82]
Fig. 9 (a,b) SEM images of Ag3PO4/GO/NiFe2 O4[82]
图10 Ag3PO4/GO/NiFe2O4的光催化机理[82]
Fig. 10 Photocatalytic mechanism of Ag3PO4/GO/NiFe2O4 composite[82]
图11 AFO/MOF/NFO的光催化机理[84]
Fig. 11 Photocatalytic mechanism of AFO/MOF/NFO[84]
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